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Single-Electron Tunneling Based Hydrogen Sensor

机译:基于单电子隧穿的氢传感器

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We present a hydrogen sensor based on single-electron tunneling in two dimensional (2D) hexagonal closed packed arrays of palladium nano-islands. The parameters of the palladium nanoparticles were extracted from the experimental TEM results by the image processing method. We also assumed random offset charges for every palladium nanoparticle. Using the SIMON simulator, the emergence of Coulomb blockade was inspected by studying the current-voltage (IV) characteristics of equivalent circuits consisting of palladium islands and tunneling junctions. After ensuring the emergence of the Coulomb blockade phenomena in these arrays, the possibilities for using these arrays as a hydrogen sensor were studied. The change in the tunneling resistances and capacitances were calculated according to the lattice parameter expansion of the palladium nanoparticles at different pressures of the hydrogen gas. The changes in the IV characteristics were investigated after exposing the arrays into hydrogen gas. The change in the resistance of the arrays before and after the exposure to hydrogen were extracted. According to the results, this configuration shows single-electron tunneling and can be used as a hydrogen gas sensor.
机译:我们目前在二维(2D)钯纳米岛的六边形密堆积阵列中基于单电子隧穿的氢传感器。通过图像处理方法从实验TEM结果中提取钯纳米粒子的参数。我们还假设了每个钯纳米粒子的随机抵消电荷。使用SIMON仿真器,通过研究由钯岛和隧道结组成的等效电路的电流-电压(IV)特性,检查了库仑阻塞的出现。在确保在这些阵列中出现库仑阻塞现象之后,研究了将这些阵列用作氢传感器的可能性。根据在不同氢气压力下钯纳米颗粒的晶格参数扩展,计算出隧穿电阻和电容的变化。将阵列暴露在氢气中后,研究了IV特性的变化。提取了暴露于氢之前和之后的阵列电阻的变化。根据结果​​,该配置显示出单电子隧穿并且可以用作氢气传感器。

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