利用分子动力学模拟方法研究了拉伸荷载作用下晶粒尺寸对纳米多晶铁变形机制的影响.研究结果表明杨氏模量随着晶粒尺寸的减小而减小.当晶粒尺寸小于15.50 nm时，纳米多晶铁的峰值应力和晶粒尺寸之间遵循反常的Hall-Petch关系，此时晶粒旋转和晶界迁移是其塑性变形的主要变形机制；随着晶粒尺寸的增大，变形孪晶和位错滑移在其塑性变形过程中逐渐占据主导地位.裂纹的形成是导致大晶粒尺寸模型力学性能降低的主要因素.纳米多晶铁在塑性变形中会出现孪晶界的迁移和退孪晶现象.此外还研究了温度对纳米多晶铁变形机制的影响.%The nanocrystalline metals are widely investigated due to their unique mechanical properties. Currently, the available studies about deformation mechanisms of metals mainly focus on face-centered cubic metals such as Ni, Cu and Au. However, the body-centered cubic metals are still very limited, despite their industrial importance. Here, we investigate the effects of grain size and temperature on the mechanical behavior of nano-polycrystalα-Fe under uniaxial tensile loading by using molecular dynamics (MD) simulation. The models of nanocrystallineα-Fe with the grain sizes of 3.95, 6.80, 9.70, 12.50, 15.50, 17.50, 20.70 and 26.00 nm are geometrically created in three dimensions by using Voronoi construction, and these models are relaxed to reach an equilibrium state. Then, each of them has a strain of 0.001 along the Z-direction in each step, keeping zero pressure in the X- and Y-directions until the strain increases up to 0.2. A 1.0 fs time step is used in all of the MD simulations. Based on the data output, the stress-strain curves at different grain sizes are obtained. The results indicate that the peak stresses of nano-polycrystalα-Fe decrease with the decrease of grain size, exhibiting a breakdown in the Hall–Petch relation when the grain size is smaller than a critical size. The major deformation mechanism is found to change from dislocation slips and twinning-mediated plasticity in a model with a larger grain size to grain boundary sliding in a model with a smaller grain size. It should be noted that twinning is formed by the emission of 1/6⟨111⟩partial dislocations along the{112}slip plane. The results show that crack formation during tension is a cause of reducing the flow stress of nano-polycrystalα-Fe with a large grain size and that the Young’s modulus of nano-polycrystal α-Fe decreases with the grain size decreasing. The main reason for the crack nucleation is here that grain boundaries perpendicular to the loading direction bear higher stress and the twin band interacts with grain boundaries at a larger grain size, causing the stress to concentrate at the intersections of grain boundaries. The results also show the detwinning behavior and migration of deformed twins in nano-polycrystal α-Fe. The detwinning behavior occurs via the migration of the intersection of grain boundary and twin, and this intersection is incoherent boundary. The migration of deformed twins proceeds by repeating initiation and glide of 1/6⟨111⟩partial dislocations on adjacent {112} planes. In addition, we find that the nucleation and propagation of dislocation become easier at higher temperature than at lower temperature.
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