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Radioactive cesium concentrations in purchased tea leaves and the other plant materials for brewing tea

机译:购买的茶叶中的放射性铯浓度和用于酿造茶的其他植物材料

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摘要

Frequently drinking tea is an ordinary custom for a large number of Japanese people. Since the radioactive cesium (Cs) in tealeaves may harm human health, the concentration should be examined as precisely as possible. In order to determine 137Cs and 134Cs concentrations, a method to isolate Cs from soil, dead leaves and leaf mold was applied for Cs isolations from green tea leaves and the other kinds of plant materials for brewing tea. Sample was carbonized in a covered stainless steel beaker (300 cm3) heated for 3 hours in an electric furnace at 450 ºC, and the Cs atoms extracted by nitric acid were collected into 1 g of ammonium phosphomolybdate trihydrate. Gamma rays from Cs sample were measured by a pure Ge detector with volume of 160 cm3 shielded by lead blocks. Results in a supplemental experiment suggested that mass reduction rate by carbonization scarcely depended on the amount of dried sample in the beaker. The Japanese products used in this study were manufactured by companies located in or western from Ibaraki prefecture. The products were obtained on or after 4 May 2013. Among 21 tea leaves products obtained for this preliminary study, the highest concentration of 137Cs was 17.8 ±0.8 Bq/kg in a product purchased in Okayama Prefecture on 28 September 2013. (The concentrations and activity ratios shown in this summary are those decay-corrected to the end of March 2011.) In this product, the 134Cs/137Cs activity ratio was 1 within uncertainty. The 137Cs concentration was as low as 0.1-0.2 Bq/kg in two Sen-tea leaves products. One was manufactured in Hyogo Prefecture and the other was manufactured in Yamaguchi Prefecture. The 137Cs concentrations in the other tea leaves products were higher than or equal to 0.3 Bq/kg. In four tea leaves products of which raw material tea leaves were produced in Shizuoka, Yamaguchi and Kagoshima Prefectures, and in two oolong tea products, the 137Cs concentrations were higher than 0.5 Bq/kg and the differences from each 134Cs concentration were 0.5 – 1.3 Bq/kg. The differences were probably caused by the 137Cs atoms emitted by the Chernobyl disaster or atmospheric nuclear weapon tests. Except tealeaves, four plant materials for brewing tea were examined in this study. The products of dried mugwort leaves for brewing tea manufactured in Oita prefecture was obtained on 26 August 2013. Both 137Cs and 134Cs concentrations in the mugwort leaves were approximately 0.4 Bq/kg. In the other three plant materials for brewing tea, both 137Cs and 134Cs concentrations were less than 0.3 Bq/kg.
机译:经常喝茶是许多日本人的习惯。由于茶叶中的放射性铯(Cs)可能危害人体健康,因此应尽可能精确地检查浓度。为了确定137Cs和134Cs的浓度,采用了从土壤,枯叶和叶片霉菌中​​分离Cs的方法,用于从绿茶叶和其他用于酿造茶的植物材料中分离Cs。将样品在带盖的不锈钢烧杯(300 cm3)中进行碳化,该烧杯在450℃的电炉中加热3小时,然后将硝酸提取的Cs原子收集到1 g三水合磷钼酸铵中。来自Cs样品的伽玛射线由纯Ge检测器测量,其中160 cm3的体积被铅块屏蔽。补充实验的结果表明,碳化引起的质量降低率几乎不依赖于烧杯中干燥样品的量。本研究中使用的日本产品由茨城县内或西部的公司生产。产品于2013年5月4日或之后获得。在本初步研究获得的21种茶叶产品中,2013年9月28日在冈山县购买的产品中137Cs的最高浓度为17.8±0.8 Bq / kg。摘要中显示的活性比是经过衰减校正到2011年3月底的活性比。)在此产品中,134Cs / 137Cs活性比在不确定范围内为1。在两种森茶叶片产品中,137Cs的浓度低至0.1-0.2 Bq / kg。一种在兵库县制造,另一种在山口县制造。其他茶叶产品中的137Cs浓度高于或等于0.3 Bq / kg。在静冈县,山口县和鹿儿岛县生产的四种以茶叶为原料的茶叶产品中,在两种乌龙茶产品中,137Cs的浓度高于0.5 Bq / kg,而每种134Cs的浓度差为0.5 – 1.3 Bq。 /公斤。造成这种差异的原因可能是切尔诺贝利灾难或大气核武器试验所发射的137Cs原子。除茶叶外,本研究还研究了四种用于冲泡茶的植物材料。 2013年8月26日,获得了大分县生产的用于冲泡茶的艾蒿干叶产品。艾蒿叶中137Cs和134Cs的浓度均约为0.4 Bq / kg。在其他三种泡茶植物材料中,137Cs和134Cs的浓度均低于0.3 Bq / kg。

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