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Detailed Structural Analysis of the Hyperbranched Polymers Formed in Self‐Condensing Vinyl Polymerization

机译：自冷凝乙烯基聚合中形成的超支化聚合物的详细结构分析

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Abstract >Monte Carlo simulation is applied to investigate the effect of reactor types on the formed hyperbranched architecture. When a continuous stirred‐tank reactor (CSTR) is used for the synthesis, the number of units incorporated into the largest cluster of dendritic units inside the hyperbranched polymer increases with molecular weight, while it does not increase in batch polymerization. The largest dendritic cluster formed in a CSTR consists of the monomeric units whose average residence time is large, while the average residence time of the singly connected peripheral units is small. The maximum span length as well as the mean‐square radius of gyration of the high molecular weight polymer is much smaller for the polymers synthesized in a CSTR, compared with batch polymerization. A universal relationship between the mean‐square radius of gyration and the maximum span length is found, which is valid for both batch and CSTR. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >蒙特卡罗模拟应用于研究反应器类型对成型超支架构的影响。当连续搅拌罐反应器（CSTR）用于合成时，结合到超支化聚合物内部的最大树枝状单位组中的单位数量随分子量而增加，同时它不会增加分批聚合。在CSTST中形成的最大树枝状簇由平均停留时间大的单体单元组成，而单个连接的外围单元的平均停留时间很小。与分批聚合相比，高分子量聚合物的最大跨度以及高分子量聚合物的聚合物的平均方形半径大得多。找到平均旋转的均方半径与最大跨度长度之间的普遍关系，这对于批次和CSTR有效。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24304/'>《Macromolecular theory and simulations》</a> <b style="margin: 0 2px;">|</b><span>2019年第2期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tobita Hidetaka&option=202" target="_blank" rel="nofollow">Tobita Hidetaka;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Materials Science and EngineeringUniversity of Fukui3‐9‐1 Bunkyo Fukui 910–8507 Japan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1185.html" title="高分子化学（高聚物）">高分子化学（高聚物）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=degree of branching&option=203" rel="nofollow">degree of branching;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hyperbranched&option=203" rel="nofollow">hyperbranched;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Monte Carlo simulation&option=203" rel="nofollow">Monte Carlo simulation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=radius of gyration&option=203" rel="nofollow">radius of gyration;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=span length&option=203" rel="nofollow">span length;</a> </p> <div class="translation"> 机译：分支学位;超支化;蒙特卡罗模拟;旋转半径;跨度长度; 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translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于进行位移/应力分析的结构分析装置，具有评价部，对详细的网格模型的分析结果进行评价，分析部取得模型的边界值，并利用该值对模型进行分析。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130453354685.html">Synthesis of multi-functional hyperbranched polymers by polymerization of di-or tri-vinyl monomers in the presence of a chain transfer catalyst</a> <b>[P]</b> . <span> 外国专利：  US5767211A </span> <span> . 1998-06-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在链转移催化剂存在下，通过二乙烯基或三乙烯基单体的聚合反应合成多功能超支化聚合物 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130461252427.html">Polymers with poly:vinyl sequences having urea di:thiocarbamate terminal gps. - made by condensing vinyl polymers with iso:cyanato di:thiocarbamate terminal gps. with di:- or poly:functional reactants</a> <b>[P]</b> . <span> 外国专利：  FR2690266A1 </span> <span> . 1993-10-22</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有聚乙烯基序列的，具有脲二氨基甲酸酯末端gps的聚合物。 -通过将乙烯基]聚合物与异氰酸酯：氰酸根合二：硫代氨基甲酸酯末端gps制成。与di：-或poly：官能反应物 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704023539071','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" 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