Organic Phototransistors Based on Self‐Assembled Microwires of n‐Type Distyrylbenzene Derivative

Lee Yoon Ho; Shin Dong‐Seon; Kim Dong Yeong; Nam Dongsik; Choe Wonyoung; Hong Sung You; Oh Joon Hak

摘要

Abstract > Molecular design and crystallinity control are important issues for the development of high‐performance organic optoelectronic devices. Here, a highly photo‐responsive n ‐type organic small molecular semiconductor, (2Z,2′Z)‐3,3′‐(2,5‐dimethoxy‐1,4‐phenylene)bis(2‐(3,5‐bis(trifluoro‐methyl)phenyl)acrylonitrile) (DM‐R), was synthesized and the photoelectronic properties of self‐assembled DM‐R microwire organic phototransistors (MW‐OPTs) were studied. Significant enhancement in the electron mobility ( μ <sub>e</sub> ) of MW‐OPTs ( μ <sub>e</sub> : 0.16?cm 2 ?V ?1 ?s ?1 ) was observed as compared to thin‐film‐OPTs ( μ <sub>e</sub> : 2.7×10 ?3 ?cm 2 ?V ?1 ?s ?1 ), most likely due to the single‐crystalline nature of the self‐assembled MWs. Moreover, the photoresponsivity of MW‐OPTs showed 23.53 (A?W ?1 ), which was 130 times higher than that of thin‐film OPTs (0.18?A?W ?1 ). Furthermore, the MW‐OPTs exhibited stable photoswitching properties and a faster charge accumulation/release rate than those of thin‐film OPTs. The results obtained herein demonstrate a facile solution‐based approach for the fabrication of high‐performance n ‐type organic MW‐OPTs and provide a systematic analysis platform of the photo‐generated charge carrier dynamics. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > 分子设计和结晶度控制是高性能有机光电器件开发的重要问题。在这里，高度光响应 n </ i> - 型有机小分子半导体，（2Z，2'Z）-3,3' - （2,5-二甲氧基-1,4-亚苯基）双（2-（3,5-双（三氟甲基）苯基）合成丙烯腈）（DM-R），研究了自组装的DM-R微针有机光电晶体管（MW-OPT）的光电性能。电子移动性的显着增强（ μ</ i> <sub> e </ sub> ）MW-OPTS（ μ</ i> <sub> e </ sub> ：0.16？cm 2 </ sup> ？V. ？1 </ sup> ？S. ？1 </ sup> 与薄膜OPTS相比，观察到）（ μ</ i> <sub> e </ sub> ：2.7×10 ？3 </ sup> ？厘米 2 </ sup> ？V. ？1 </ sup> ？S. ？1 </ sup> ），很可能是由于自组装MWS的单晶性质。此外，MW-OPTS的光反对子显示显示23.53（a？w ？1 </ sup> ），比薄膜OPTS高130倍（0.18？a？w ？1 </ sup> ）。此外，MW-opts表现出稳定的光学开养性能，比薄膜选择速度更快的电荷累积/释放速率。本文获得的结果表明了用于制备高性能的基于溶液的方法 n </ i> -Type有机MW-OPTS并提供光生成的电荷载体动态的系统分析平台。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19765/'>《Asian Journal of Organic Chemistry》</a> <b style="margin: 0 2px;">|</b><span>2018年第11期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Yoon Ho&option=202" target="_blank" rel="nofollow">Lee Yoon Ho;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shin Dong‐Seon&option=202" target="_blank" rel="nofollow">Shin Dong‐Seon;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Dong Yeong&option=202" target="_blank" rel="nofollow">Kim Dong Yeong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nam Dongsik&option=202" target="_blank" rel="nofollow">Nam Dongsik;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Choe Wonyoung&option=202" target="_blank" rel="nofollow">Choe Wonyoung;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hong Sung You&option=202" target="_blank" rel="nofollow">Hong Sung You;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Oh Joon Hak&option=202" target="_blank" rel="nofollow">Oh Joon Hak;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Chemical and Biological Engineering Institute of Chemical ProcessesSeoul National University1 Gwanak-ro Seoul 08826 Republic of Korea;</p> <p>School of Energy and Chemical EngineeringUlsan National Institute of Science and Technology (UNIST)50 UNIST-gil Ulsan 44919 Republic of Korea;</p> <p>School of Chemical and Biological Engineering Institute of Chemical ProcessesSeoul National University1 Gwanak-ro Seoul 08826 Republic of Korea;</p> <p>Department of ChemistryUNIST50 UNIST-gil Ulsan 44919 Republic of Korea;</p> <p>Department of ChemistryUNIST50 UNIST-gil Ulsan 44919 Republic of Korea;</p> <p>School of Energy and Chemical EngineeringUlsan National Institute of Science and Technology (UNIST)50 UNIST-gil Ulsan 44919 Republic of Korea;</p> <p>School of Chemical and Biological Engineering Institute of Chemical ProcessesSeoul National University1 Gwanak-ro Seoul 08826 Republic of Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1184.html" title="有机化学">有机化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Photo-responsive materials&option=203" rel="nofollow">Photo-responsive materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=organic semiconductors&option=203" rel="nofollow">organic semiconductors;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=microwires&option=203" rel="nofollow">microwires;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=1-D materials&option=203" rel="nofollow">1-D materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=organic phototransistors&option=203" rel="nofollow">organic phototransistors;</a> </p> <div class="translation"> 机译：光响应材料;有机半导体;微挖;1-D材料;有机光电晶体管; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022774305.html">Organic Phototransistors Based on Self‐Assembled Microwires of n‐Type Distyrylbenzene Derivative</a> <b>[J]</b> . 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