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Graphene Oxide Induced High Crystallinity of SAPO‐11 Molecular Sieves for Improved Alkane Isomerization Performance

机译：石墨烯氧化物诱导SAPO-11分子筛的高结晶度，以改善烷烃异构化性能

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Abstract >In the presence of graphene oxide (GO), highly crystallized SAPO‐11 molecular sieves were prepared by a non‐solvent method. The functional groups of GO bind with raw materials, with the formation of hydrogen bonds and acid amides, verified by the XPS analysis. The inorganic precursor and structure‐directing agent molecules will be fixed on the surface of GO, increasing the reaction rate and crystallization for SAPO‐11 preparation, confirmed by the XRD and BET results. Meanwhile, the IR analysis of the adsorption of pyridine indicates there are more acidic sites for the highly crystallized SAPO‐11 sample. The resultant well‐crystallized SAPO‐11 molecular sieves exhibited greater isomer yield and better catalytic activity compared to traditional SAPO‐11 prepared without GO. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 在氧化石墨烯（GO）的存在下，通过非溶剂方法制备高度结晶的SAPO-11分子筛。通过XPS分析形成氢键和酸酰胺的形成与原料的官能团。无机前体和结构引导剂分子将固定在去的表面上，增加SAPO-11制剂的反应速率和结晶，通过XRD和BET结果证实。同时，对吡啶吸附的红外分析表明高度结晶的SAPO-11样品有更多的酸性位点。与传统的SAPO-11相比，所得良好结晶的SAPO-11分子筛表现出更大的异构体产量和更好的催化活性，而无需进行。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16168/'>《ChemNanoMat》</a> <b style="margin: 0 2px;">|</b><span>2019年第9期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Yanyan&option=202" target="_blank" rel="nofollow">Du Yanyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yao Heliang&option=202" target="_blank" rel="nofollow">Yao Heliang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Lei&option=202" target="_blank" rel="nofollow">Zhao Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Hongmei&option=202" target="_blank" rel="nofollow">Yang Hongmei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Min&option=202" target="_blank" rel="nofollow">Wang Min;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yuan Long&option=202" target="_blank" rel="nofollow">Yuan Long;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Yanhui&option=202" target="_blank" rel="nofollow">Xu Yanhui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Jiusheng&option=202" target="_blank" rel="nofollow">Li Jiusheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Green Chemical Engineering Technology Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210 P. R. China;</p> <p>Analysis &</p> <p>Testing Center for Inorganic Materials Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050 P. R. China;</p> <p>Green Chemical Engineering Technology Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210 P. R. China;</p> <p>Green Chemical Engineering Technology Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210 P. R. China;</p> <p>College of Materials Science &</p> <p>EngineeringQingdao University of Science &</p> <p>Technology53 Zhengzhou Road Qingdao 266042 P. R. China;</p> <p>Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of EducationJilin Normal UniversityChangchun P. R. China;</p> <p>Green Chemical Engineering Technology Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210 P. R. China;</p> <p>Green Chemical Engineering Technology Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1676.html" title="工程材料学">工程材料学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=bifunctional catalysts&option=203" rel="nofollow">bifunctional catalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=high crystallinity&option=203" rel="nofollow">high crystallinity;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene oxide&option=203" rel="nofollow">graphene oxide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydroisomerization&option=203" rel="nofollow">hydroisomerization;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=non-solvent method&option=203" rel="nofollow">non-solvent method;</a> </p> <div class="translation"> 机译：双官能催化剂;高结晶度;石墨烯氧化物;加氢异构化;非溶剂方法; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022088762.html">Graphene Oxide Induced High Crystallinity of SAPO‐11 Molecular Sieves for Improved Alkane Isomerization Performance</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Yanyan&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Du Yanyan,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yao Heliang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yao Heliang,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Lei&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhao Lei,</a> <a href="/journal-foreign-16168/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemNanoMat .</a> <span>2019</span><span>,第9期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：石墨烯氧化物诱导SAPO-11分子筛的高结晶度，以改善烷烃异构化性能</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704014006658.html">Impact of cationic surfactant chain length during SAPO-11 molecular sieve synthesis on structure, acidity, and n-octane isomerization to di-methyl hexanes</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo L.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Guo L.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bao X.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Bao X.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fan Y.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Fan Y.,</a> <a href="/journal-foreign-34045/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Catalysis .</a> <span>2012</span><span>,第Null期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：SAPO-11分子筛合成过程中阳离子表面活性剂链长对结构，酸度和正辛烷异构化为二甲基己烷的影响</span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/070403007008.html">1-pentene isomerization over SAPO-11, BEA and A1MCM-41 molecular sieves</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lopez CM&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Lopez CM,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ramirez L&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ramirez L,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sazo V&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Sazo V,</a> <a href="/journal-foreign-19278/" target="_blank" rel="nofollow" class="tuijian_authcolor">Applied Catalysis, A. 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href="/academic-journal-cn_journal-fuel-chemistry-technology_thesis/0201247867466.html">乙醇对Pt/SAPO-11和Pt/ZSM-22催化剂烷烃异构化性能的影响</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=柴志波&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 柴志波</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=吕恩静&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,吕恩静</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张怀科&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张怀科</a> <span> <a href="/journal-cn-9180/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 燃料化学学报 </a> </span> <span> . 2014</span><span>,第002期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-8497_thesis/020222151440.html">SAPO-11分子筛上长链烷烃异构化研究进展</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=靳丽丽&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 靳丽丽</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王新苗&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王新苗</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=孟祥斌&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,孟祥斌</a> <span> <a href="/conference-cn-8497/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第九届全国工业催化技术及应用年会 </a> <span> <span> . 2012</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314127814.html">Ⅰ.SAPO-11分子筛上长链烷烃异构化性能研究;Ⅱ.TS-1分子筛的合成及其苯酚氧化反应性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=邓鹏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 邓鹏</a> <span> . 2000</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120112523830.html">一种多级孔SAPO-11分子筛及长链烷烃异构化催化剂的制备方法与应用</a> <b>[P]</b> . <span> 中国专利： CN112536067A </span> <span> . 2021-03-23</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061202912338.html">一种高结晶度SAPO-11分子筛的制备方法</a> <b>[P]</b> . <span> 中国专利： CN105668589B </span> <span> . 2018.06.29</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130430305308.html">AN IMPROVED PROCESS FOR PREPARATION OF CRYSTALLINE SAPO -11 TYPE NON-ZEOLITIC MOLECULAR SIEVE</a> <b>[P]</b> . <span> 外国专利：  IN224644B </span> <span> . 2008-12-05</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：结晶SAPO -11型非沸石分子筛的制备工艺改进 </span> </p> </li> <li> <div> <b>4. </b><a 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