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Multipolar second harmonic generation in a symmetric nonlinear metamaterial

机译:对称非线性超材料中的多极二次谐波产生

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摘要

Optical nonlinearities are intimately related to the spatial symmetry of the nonlinear media. For example, the second order susceptibility vanishes for centrosymmetric materials under the dipole approximation. The latter concept has been naturally extended to the metamaterials’ realm, sometimes leading to the (erroneous) hypothesis that second harmonic (SH) generation is negligible in highly symmetric meta-atoms. In this work we aim to show that such symmetric meta-atoms can radiate SH light efficiently. In particular, we investigate in-plane centrosymmetric meta-atom designs where the approximation for meta-atoms breaks down. In a periodic array this building block allows us to control the directionality of the SH radiation. We conclude by showing that the use of symmetry considerations alone allows for the manipulation of the nonlinear multipolar response of a meta-atom, resulting in e.g. dipolar, quadrupolar, or multipolar emission on demand. This is because the size of the meta-atom is comparable with the free-space wavelength, thus invalidating the dipolar approximation for meta-atoms.
机译:光学非线性与非线性介质的空间对称性密切相关。例如,在偶极近似下,中心对称材料的二阶磁化率消失。后者的概念已自然地扩展到超材料的领域,有时会导致(错误的)假设,即在高对称的超原子中,二次谐波(SH)的产生可以忽略。在这项工作中,我们旨在证明这种对称的亚原子可以有效地辐射SH光。特别是,我们研究平面内中心对称的亚原子设计,其中亚原子的近似分解。在一个周期性阵列中,该构造块使我们能够控制SH辐射的方向性。我们通过显示得出结论,仅使用对称性考虑因素就可以操纵一个亚原子的非线性多极响应,从而导致例如按需提供双极,四极或多极发射。这是因为准原子的大小与自由空间波长相当,因此使准原子的偶极近似无效。

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