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Artificial kagome spin ice.

机译:人造kagome旋转冰。

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摘要

Geometrical frustration is known to significantly modify the properties of many materials. Pyrochlore spin ice and hexagonal water ice are canonical systems that show the effects of frustration in both heat capacity and dynamical response. In both instances, microscopic ordering principles on the lattice lead to a macroscopic degeneracy of configurations. This degeneracy in spin ice may also be modified or lifted by lattice imperfections, external pressure, or magnetic field. Unfortunately, these effects are difficult to model or predict, because existing experimental techniques cannot directly observe the local ordering, near lattice defects or otherwise. To address this long outstanding problem, recent interest has focused on fabricating systems that allow the effects of frustration to be physically modeled and the resulting local configurations to be directly observed.;In this dissertation, I present an artificial approach to kagome lattice. The kagome lattice is a two-dimensional structure composed of corner-sharing triangles and is an essential component of the pyrochlore spin ice structure. Our artificial kagome spin ice, constructed by magnetic nano-bar elements, mimics spin ice in 2D. The realized system rigorously obeys the ice rule (2-in 1-out or 1-in 2-out configuration at a vertex of three elements), thus providing a sought-after model system appropriate for further studies.;To study the ground state of the artificial kagome system and to validate the artificial approach for spin ice study, we demagnetize the samples using rotating field and observe spin configurations using Lorentz TEM. The ice rule, short-range ordering and absence of long-range disorder, as well as the relatively low remnant magnetization are found in the system, which are signatures of spin ice materials in their ground states. To model our system and relate it to other spin study, we introduce magnetic charge model and Shannon entropy concept. The calculated charge correlation (charge ordering coefficient) and Shannon entropy suggest that the degeneracy of our lattice is lifted from a completely disordered kagome spin ice system, and close to a "true" ground state that is usually found as the kagome plateau in pyrochlore spin ice when applying a field in 111> direction.;We also study the effects of external perturbations. When applying a magnetic field, chain-like spin flipping is found in the system, which can be explained by the magnetic charge model. When distorting the lattice by introducing an artificial strain, we observe partial ordering or symmetry breaking in the system, which is similar to the pressure effects in real spin ice.;In the Appendix, I also introduce another study I have done, i.e. multiferroic thin film measurements. The focus of that chapter is the dielectric measurement for BaTiO3 (BTO) -CoFe2O4 (CFO) thin film material using a microwave microscope. The measurement has a quantitative spatial resolution of approximately 5 microm, and it provides a method for film quality check and the basis for a proposed ME coupling measurement.
机译:众所周知,几何挫折会极大地改变许多材料的性能。烧绿石自旋冰和六角形水冰是典范的系统,在热容量和动力响应方面均表现出挫折感。在这两种情况下,晶格上的微观排序原理都会导致结构的宏观退化。旋转冰中的这种简并性还可以通过晶格缺陷,外部压力或磁场来改变或消除。不幸的是,这些效果很难建模或预测,因为现有的实验技术无法直接观察局部有序,接近晶格缺陷或其他情况。为了解决这个长期存在的问题,最近的兴趣集中在制造系统上,该系统可以对挫折的影响进行物理建模,并可以直接观察到产生的局部结构。;在本文中,我提出了一种人工方法来构造kagome晶格。 kagome晶格是由角共享三角形组成的二维结构,并且是烧绿石自旋冰结构的重要组成部分。我们的人造kagome旋转冰由磁性纳米棒元件构成,可模拟二维旋转冰。所实现的系统严格遵守冰规则(在三个元素的顶点处2进1出或1进2出配置),从而为以后的研究提供了一种受欢迎的模型系统。人造kagome系统的原理,并验证用于旋转冰研究的人工方法,我们使用旋转磁场对样品进行消磁,并使用Lorentz TEM观察旋转结构。在系统中发现了冰规则,短程有序性和远距离无序性以及相对较低的剩余磁化强度,这是自旋冰材料在其基态下的特征。为了建模我们的系统并将其与其他自旋研究联系起来,我们引入了磁电荷模型和香农熵概念。计算出的电荷相关性(电荷有序系数)和香农熵表明,我们晶格的简并性是从完全无序的kagome自旋冰系统中解脱出来的,并且接近于“真”基态,通常在烧绿石自旋中作为kagome高原被发现。在<111>方向施加磁场时会结冰。;我们还研究了外部扰动的影响。当施加磁场时,在系统中会发现链状自旋翻转,这可以用磁电荷模型来解释。当通过引入人工应变使晶格变形时,我们会观察到系统中的部分有序排列或对称破坏,这与真实自旋冰中的压力效应相似。;在附录中,我还介绍了我所做的另一项研究,即多铁性薄电影测量。该章的重点是使用微波显微镜对BaTiO3(BTO)-CoFe2O4(CFO)薄膜材料进行介电测量。该测量具有大约5微米的定量空间分辨率,它为薄膜质量检查提供了一种方法,并为提出的ME耦合测量提供了基础。

著录项

  • 作者

    Qi, Yi.;

  • 作者单位

    University of Maryland, College Park.;

  • 授予单位 University of Maryland, College Park.;
  • 学科 Physics Condensed Matter.;Engineering Materials Science.
  • 学位 Ph.D.
  • 年度 2008
  • 页码 129 p.
  • 总页数 129
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 工程材料学;
  • 关键词

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