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Multipolar analysis of second-harmonic generation in GaAs nanoparticles grown along different crystallographic directions

机译:沿不同晶体方向生长的GaAs纳米粒子二次谐波发电的多极化分析

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We perform multipolar analysis of second-harmonic generation (SHG) from gallium arsenide (GaAs) nanoantennas grown along different crystallographic directions and discuss their specifics. In particular, analysis of the nonlinear response of nanoantennas grown along the (110) axis based on the Lorentz lemma shows that such nanoantennas generate multipoles with only odd azimuthal index m. This feature of (110)-GaAs nanoantennas provides the best forward/backward directivity as compared to their (100) and (111) counterparts. Using numerical modeling we determine parameters of the cylindrical nanoantenna to achieve optical switching in the nonlinear regime by rotating the pump polarization. We then experimentally demonstrate the nonlinear switching between forward and backward SHG emissions from (110)-grown GaAs nanodisks.
机译:我们从沿不同的晶体方向生长的砷化镓(GaAs)纳米纳拉斯的二极管发电(SHG)的多极分析,并讨论其细节。 特别地,沿着Lorentz Lemma沿(110)轴生长的纳米环的非线性响应的分析表明,这种纳米环绕具有仅具有奇数方位角指数m的多孔。 (110)-GAAS纳米宁纳米的这种特征提供与(100)和(111)对应相比的最佳前向/后向方向性。 使用数值模拟我们通过旋转泵极化来确定圆柱形纳米纳尼纳的参数,以通过旋转泵极化实现非线性状态的光学切换。 然后,我们通过(110)-110)-BlownAnodisks进行了实验地展示了前向和落后的SHG排放之间的非线性切换。

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