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Decoherence and fluctuation dynamics of the quantum dot nuclear spin bath probed by nuclear magnetic resonance

机译:核磁共振探测量子点核自旋浴的消相干和波动动力学

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摘要

Dynamics of nuclear spin decoherence and nuclear spin flip-flops in self-assembled InGaAs/GaAs quantum dots are studied experimentally using optically detected nuclear magnetic resonance (NMR). Nuclear spin-echo decay times are found to be in the range 1-4 ms. This is a factor of ~3 longer than in strain-free GaAs/AlGaAs structures and is shown to result from strain-induced quadrupolar effects that suppress nuclear spin flip-flops. The correlation times of the flip-flops are examined using a novel frequency-comb NMR technique and are found to exceed 1 s, a factor of ~1000 longer than in strain-free structures. These findings complement recent studies of electron spin coherence and reveal the paradoxical dual role of the quadrupolar effects in self-assembled quantum dots: large increase of the nuclear spin bath coherence and at the same time significant reduction of the electron spin-qubit coherence. Approaches to increasing electron spin coherence are discussed. In particular the nanohole filled GaAs/AlGaAs quantum dots are an attractive option: while their optical quality matches the self-assembled dots the quadrupolar effects measured in NMR spectra are a factor of 1000 smaller.
机译:使用光学检测的核磁共振(NMR),通过实验研究了自组装InGaAs / GaAs量子点中核自旋退相干和核自旋触发器的动力学。发现核自旋回波衰减时间在1-4ms的范围内。这比无应变的GaAs / AlGaAs结构长约3倍,并且显示是由于应变引起的四极效应而抑制核自旋触发器。使用新颖的频率梳NMR技术检查触发器的相关时间,发现它们超过1 s,比无应变结构长约1000倍。这些发现补充了对电子自旋相干的最新研究,并揭示了四极效应在自组装量子点中的悖论双重作用:核自旋浴相干性的大幅提高,同时电子自旋量子位相干性的显着降低。讨论了提高电子自旋相干性的方法。尤其是,纳米孔填充的GaAs / AlGaAs量子点是一个有吸引力的选择:尽管它们的光学质量与自组装点匹配,但在NMR光谱中测得的四极效应小了1000倍。

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    Chekhovich E.A.;

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  • 年度 2017
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  • 原文格式 PDF
  • 正文语种 en
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