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Mixing of dust and NH3 observed globally over anthropogenic dust sources

机译:在人为的粉尘源上观察到的粉尘与NH3的混合

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摘要

The global distribution of dust column burden derived from MODIS Deep Blueaerosol products is compared to NH column burden retrieved from IASIinfrared spectra. We found similarities in their spatial distributions, inparticular their hot spots are often collocated over croplands and to alesser extent pastures. Globally, we found 22% of dust burdencollocated with NH, with only 1% difference between land-usedatabases. This confirms the importance of anthropogenic dust fromagriculture. Regionally, the Indian subcontinent has the highest amount ofdust mixed with NH (26%), mostly over cropland and during thepre-monsoon season. North Africa represents 50% of total dust burden butaccounts for only 4% of mixed dust, which is found over croplands andpastures in Sahel and the coastal region of the Mediterranean. In order toevaluate the radiative effect of this mixing on dust optical properties, wederive the mass extinction efficiency for various mixtures of dust andNH, using AERONET sunphotometers data. We found that for dusty daysthe coarse mode mass extinction efficiency decreases from 0.62 to0.48 m g as NH burden increases from 0 to 40 mg m.The fine mode extinction efficiency, ranging from 4 to 16 m g,does not appear to depend on NH concentration or relative humidity butrather on mineralogical composition and mixing with other aerosols. Ourresults imply that a significant amount of dust is already mixed withammonium salt before its long range transport. This in turn will affect dustlifetime, and its interactions with radiation and cloud properties.
机译:将来自MODIS深蓝气溶胶产品的粉尘柱负荷的全球分布与从IASI红外光谱中检索到的NH柱负荷进行比较。我们发现它们的空间分布有相似之处,尤其是它们的热点通常分布在农田和较小范围的牧场上。在全球范围内,我们发现22%的粉尘负担与NH并存,而土地利用数据库之间只有1%的差异。这证实了来自农业的人为扬尘的重要性。在区域上,印度次大陆的粉尘与NH混合量最高(26%),主要分布在农田和季风前季节。北非占尘埃总负担的50%,但仅占混合尘埃的4%,这是在萨赫勒地区和地中海沿岸地区的农田和草场中发现的。为了评估这种混合对粉尘光学性能的辐射影响,使用AERONET日光光度计数据,推导了粉尘和NH的各种混合物的质量消光效率。我们发现在尘土飞扬的日子里,随着NH的负荷从0增加到40 mg / m,粗模式的消光效率从0.62降低到0.48 mg.4到16 mg的精细模式的消光效率似乎与NH的浓度无关或相对湿度反而对矿物组成和与其他气溶胶混合。我们的结果表明,在远距离运输之前,大量的粉尘已经与铵盐混合。反过来,这将影响粉尘寿命,及其与辐射和云特性的相互作用。

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