The response of thermally and optically stimulated luminescence from Al2O3 : C to high-energy heavy charged particles

摘要

The thermoluminescence (TL) and optically stimulated luminescence (OSL) response of Al2O3 dosimeters to high-energy heavy charged particles (HCP) has been studied using the heavy ion medical accelarator at Chiba, Japan. The samples were Al2O3 single-crystal chips, of the type usually known as TLD-500, and Luxel(TM) dosimeters (Al2O3:C powder in plastic) from Landauer Inc. The samples were exposed to He-4 (150 MeV/u), C-12 (400 MeV/u), Si-28 (490 MeV/u) and 16 Fe (500 MeV/u) ions, with linear energy transfer values covering the range from 2.26 to 189 keV/mum in water and doses from I to 100 mGy (to water). A Sr-90/Y-90 beta source, calibrated against a Co-60 secondary standard, was used for calibration purposes. For OSL, we used both continuous-wave OSL measurements (CW-OSL, using green light stimulation at 525 nm) and pulsed OSL measurements (POSL, using 532 nm stimulation from a Nd:YAG Q-switched laser). The efficiencies (eta(HCP,y)) of the different HCPs at producing OSL or TL were observed to depend not only upon the linear energy transfer (LET) of the HCP, but also upon the sample type (single crystal chip or Luxel(TM)) and the luminescence method used to define the signal-i.e. TL, CW-OSL initial intensity, CW-OSL total area, or POSL. Observed changes in shape of the decay curve lead to potential methods for extracting LET information of unknown radiation fields. A discussion of the results is given, including the potential use of OSL from Al2O3 in the areas of space radiation dosimetry and radiation oncology. (C) 2004 Elsevier Ltd. All rights reserved.