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首页> 外文期刊>Angewandte Chemie >Crystal‐Growth‐Dominated Fabrication of Metal–Organic Frameworks with Orderly Distributed Hierarchical Porosity
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Crystal‐Growth‐Dominated Fabrication of Metal–Organic Frameworks with Orderly Distributed Hierarchical Porosity

机译：用有序分布的分层孔隙率的金属 - 有机框架的晶体生长主导的制造

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Abstract >Constructing architectures with hierarchical porosity has been widely considered as the most efficient way to bypass the problems related to slow mass transfer and inaccessibility of internal space in MOFs. Now, a crystal‐growth‐dominated strategy is proposed to fabricate hierarchically porous MOFs (HP‐MOFs). When the crystal growth is dominated by the monomer attachment, the aggregation of nonionic surfactant or polymer can be easily captured and released during the crystal growth process, resulting in the formation and ordering hierarchical pores along the radial direction. Owing to the accelerated mass diffusion and more exposed active sites of this design, HP‐MOFs exhibited an enhanced catalytic efficiency in styrene oxidation. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >构建具有层级孔隙度的架构已被广泛认为是绕过与MOF中内部空间缓慢传输相关问题的最有效方式。 现在，提出了一种晶体生长束缚的策略来制造分层多孔MOF（HP-MOF）。 当晶体生长由单体附着主导时，可以在晶体生长过程中容易地捕获并释放聚合物的聚集，导致沿径向形成和排序分级孔。 由于加速的质量扩散和这种设计的更暴露的活性位点，HP-MOF在苯乙烯氧化中表现出增强的催化效率。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第6期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Hang&option=202" target="_blank" rel="nofollow">Li Hang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Meng Fanchen&option=202" target="_blank" rel="nofollow">Meng Fanchen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Suoying&option=202" target="_blank" rel="nofollow">Zhang Suoying;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Liguang&option=202" target="_blank" rel="nofollow">Wang Liguang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Matthew&option=202" target="_blank" rel="nofollow">Li Matthew;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Lu&option=202" target="_blank" rel="nofollow">Ma Lu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Weina&option=202" target="_blank" rel="nofollow">Zhang Weina;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Wenlei&option=202" target="_blank" rel="nofollow">Zhang Wenlei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Zhuhong&option=202" target="_blank" rel="nofollow">Yang Zhuhong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Tianpin&option=202" target="_blank" rel="nofollow">Wu Tianpin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Sungsik&option=202" target="_blank" rel="nofollow">Lee Sungsik;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huo Fengwei&option=202" target="_blank" rel="nofollow">Huo Fengwei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Jun&option=202" target="_blank" rel="nofollow">Lu Jun;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Materials-Oriented Chemical EngineeringNanjing Tech UniversityNanjing 210009 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) &</p> <p>Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) &</p> <p>Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>X-ray Sciences DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> <p>Chemical Sciences and Engineering DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> <p>X-ray Sciences DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) &</p> <p>Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) &</p> <p>Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>State Key Laboratory of Materials-Oriented Chemical EngineeringNanjing Tech UniversityNanjing 210009 P. R. China;</p> <p>X-ray Sciences DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> <p>X-ray Sciences DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> <p>Key Laboratory of Flexible Electronics (KLOFE) &</p> <p>Institute of Advanced Materials (IAM)Nanjing Tech University30 South Puzhu Road Nanjing 211816 P. R. China;</p> <p>Chemical Sciences and Engineering DivisionArgonne National LaboratoryLemont IL 60439 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crystal growth&option=203" rel="nofollow">crystal growth;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchical porosity&option=203" rel="nofollow">hierarchical porosity;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal–organic frameworks&option=203" rel="nofollow">metal–organic frameworks;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanostructures&option=203" rel="nofollow">nanostructures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=styrene&option=203" rel="nofollow">styrene;</a> </p> <div class="translation"> 机译：晶体生长;层次结构;金属有机框架;纳米结构;苯乙烯; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028162440.html">Crystal‐Growth‐Dominated Fabrication of Metal–Organic Frameworks with Orderly Distributed Hierarchical Porosity</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Hang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Li Hang,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Meng Fanchen&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Meng Fanchen,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Suoying&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhang Suoying,</a> <a href="/journal-foreign-19011/" target="_blank" rel="nofollow" class="tuijian_authcolor">Angewandte Chemie .</a> <span>2020</span><span>,第6期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用有序分布的分层孔隙率的金属 - 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<span> . 2016</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061203369303.html">一种有序大孔金属有机框架单晶及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN107629076B </span> <span> . 2019.06.18</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120101250619.html">利用金属有机框架制备三维有序分级多孔碳光子晶体方法</a> <b>[P]</b> . <span> 中国专利： CN110407192A </span> <span> . 2019-11-05</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130414375753.html">Mesoporous metal-organic frameworks with dominating interparticular porosity, methods for preparation thereof and uses</a> <b>[P]</b> . <span> 外国专利： <!-- 欧洲知识产权局专利： --> EP2878366A1 </span> <span> . 2015-06-03</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有主要的颗粒间孔隙的中孔金属有机骨架，其制备方法和用途 </span> 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COMPOSITE</a> <b>[P]</b> . <span> 外国专利： <!-- 美国专利： --> US2017072383A1 </span> <span> . 2017-03-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含在主体金属有机框架中的纳米金属有机框架的金属有机框架复合材料，制备金属有机框架复合材料的方法和包括金属有机框架复合材料的气体存储 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704028162440','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> 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