<![CDATA[Sodium vanadium nitridophosphate Na <ce:inf loc='post'>3</ce:inf>V(PO <ce:inf loc='post'>3</ce:inf>) <ce:inf loc='post'>3</ce:inf>N as a high-voltage positive electrode material for Na-ion and Li-ion batteries]]>

Marine Reynaud; Agnieszka Wizner; Nebil A. Katcho; Laura C. Loaiza; Montserrat Galceran; Javier Carrasco; Teófilo Rojo; Michel Armand; Montse Casas-Cabanas

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3V(PO 3) 3N as a high-voltage positive electrode material for Na-ion and Li-ion batteries]]>

机译：<！[CDATA [CDATA [钒硝基磷酸钠NA 3 V（PO 3 ） 3 n作为NA-ION和LI-ION电池的高压正极材料]]]>

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Abstract

We report the preparation and electrochemical properties of Na3V(PO3)3N made by ammonolysis. Na3V(PO3)3N is reversibly oxidized to Na2V(PO3)3N at high voltage (4.0Vvs. Na+/Na0and 4.1Vvs. Li+/Li0) with an unusually small difference in the insertion/extraction voltage between both alkali metal reference electrodes. In both cases, the voltage hysteresis is extremely small (~0.035Vvs. sodium and ~0.065Vvs. lithium), which suggests facile migration of alkali cations within the structure. Further oxidation to NaV(PO3)3N is predicted to occur beyond the voltage stability window of the electrolytes.

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我们报告NA 3 V（PO 3 ） 3 N由氨解制。 NA 3 V（PO 3 ） 3 n可逆地被氧化为na 2 v（po 3 ） 3 N，高电压（4.0V 与。NA + < / ce：sup> / na 0 和4.1v vs 。li + / li 0 ）在碱金属参考电极之间的插入/提取电压具有异常小的差异。在这两种情况下，电压滞后极小（〜0.035V Vs 。钠和〜0.065V 与。锂），这表明碱阳离子在结构内的裂缝迁移。进一步氧化到NAV（PO 3 ） 3 n超出电压稳定性电解质的窗口。

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来源
《Electrochemistry communications》 |2017年第2017期|共5页
作者
Marine Reynaud; Agnieszka Wizner; Nebil A. Katcho; Laura C. Loaiza; Montserrat Galceran; Javier Carrasco; Teófilo Rojo; Michel Armand; Montse Casas-Cabanas;
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作者单位

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

CIC energiGUNE Parque Tecnológico de álava;

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原文格式 PDF
正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
关键词
Li-ion batteries; Na-ion batteries; Positive electrode material; Cathode; Nitridophosphate;

机译：锂离子电池;Na离子电池;正极材料;阴极;硝基磷酸盐;
入库时间 2022-08-20 02:37:03

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3V(PO 3) 3N as a high-voltage positive electrode material for Na-ion and Li-ion batteries]]>

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