Decoration of Nanofibrous Paper Chemiresistors with Dendronized Nanoparticles toward Structurally Tunable Negative‐Going Response Characteristics to Human Breathing and Sweating

Yan Shan; Liu Xin; Skeete Zakiya; He Ning; Xie Zhi‐Hui; Zhao Wei; Lombardi Jack P.; Liu Kai; Kang Ning; Luo Jin; Hsiao Benjamin S.; Poliks Mark; Gitsov Ivan; Zhong Chuan‐Jian

摘要

Abstract >The development of wearable breath or sweat sensor arrays for human performance monitoring is increasingly important for providing personalized health information under various environmental conditions. A major challenge is the lack of sensing elements responsive uniquely to moisture‐dominated breathing and sweating processes, which is critical for differentiating other chemical or biological species from the moisture‐dominated environment. Here a novel class of nanofibrous paper chemiresistors decorated with dendronized nanoparticles that exhibit structurally tunable and negative‐going responses to human breathing and sweating is reported. The nanocomposite device features flexible membrane‐type scaffold derived from multilayered nanofibrous paper as a biocompatible matrix and dendronized gold nanoparticles with tunable sizes and shapes to enable structural diversity and molecular sensitivity. Key elements of novelty include the immobilization of poly(ether‐ester) dendrons with oligoethylene glycol spacers on gold nanoparticles and the combination of hydrogen bonding and van der Waals interactions between partially interpenetrating dendrons, leading to tunable and unique response characteristics to breathing and sweating processes. The results demonstrate the first example of nanofibrous paper chemiresistors decorated with dendronized nanoparticles as a promising new strategy toward constructing sensing interfaces for wearable breath and sweat sensors. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >人类性能监测的可穿透呼吸或汗水传感器阵列对于在各种环境条件下提供个性化健康信息越来越重要。一项重大挑战是缺乏对湿气占呼吸和出汗过程的响应性的传感元素，这对于区分其他化学品或生物物种来与水分占主导地位的环境至关重要。在这里，一种新型的纳米纤维化学体化学，据报道，纳米颗粒纳米颗粒，其表现出对人类呼吸和出汗的结构可调和负面的反应。纳米复合装置具有源自多层纳米纤维纸的柔性膜型支架作为生物相容性基质和具有可调谐尺寸和形状的树枝状金纳米粒子，以实现结构分集和分子敏感性。新奇的关键要素包括在金纳米颗粒上与寡甘醇醇间隔物固定聚（醚酯）树枝状物，氢键和van der Wa的组合与部分互穿树枝状的相互作用，导致呼吸和出汗过程的可调和独特的响应特性。结果表明，纳米纤维纸化学电池的第一例用树木化纳米颗粒装饰为一个有希望的新策略，旨在构建可穿戴呼吸和汗水传感器的传感界面。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第22期</span><b style="margin: 0 2px;">|</b><span>共11页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Shan&option=202" target="_blank" rel="nofollow">Yan Shan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Xin&option=202" target="_blank" rel="nofollow">Liu Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Skeete Zakiya&option=202" target="_blank" rel="nofollow">Skeete Zakiya;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Ning&option=202" target="_blank" rel="nofollow">He Ning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xie Zhi‐Hui&option=202" target="_blank" rel="nofollow">Xie Zhi‐Hui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Wei&option=202" target="_blank" rel="nofollow">Zhao Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lombardi Jack P.&option=202" target="_blank" rel="nofollow">Lombardi Jack P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Kai&option=202" target="_blank" rel="nofollow">Liu Kai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kang Ning&option=202" target="_blank" rel="nofollow">Kang Ning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Luo Jin&option=202" target="_blank" rel="nofollow">Luo Jin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hsiao Benjamin S.&option=202" target="_blank" rel="nofollow">Hsiao Benjamin S.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Poliks Mark&option=202" target="_blank" rel="nofollow">Poliks Mark;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gitsov Ivan&option=202" target="_blank" rel="nofollow">Gitsov Ivan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhong Chuan‐Jian&option=202" target="_blank" rel="nofollow">Zhong Chuan‐Jian;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of ChemistryState University of New York‐ESFSyracuse NY 13210 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of Chemical and Biochemical EngineeringXiamen UniversityXiamen 361005 China;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of ChemistryStony Brook UniversityStony Brook NY 11794 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of ChemistryStony Brook UniversityStony Brook NY 11794 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> <p>Department of ChemistryState University of New York‐ESFSyracuse NY 13210 USA;</p> <p>Department of Chemistry and System Science and Industrial EngineeringState University of New York at BinghamtonBinghamton NY 13902 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=breath sensor&option=203" rel="nofollow">breath sensor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dendronized gold nanoparticles&option=203" rel="nofollow">dendronized gold nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanofibrous membrane paper&option=203" rel="nofollow">nanofibrous membrane paper;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sweat sensor&option=203" rel="nofollow">sweat sensor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=tunable nanocomposite interfaces&option=203" rel="nofollow">tunable nanocomposite interfaces;</a> </p> <div class="translation"> 机译：呼吸传感器;Dendronized金纳米颗粒;纳米纤维膜;汗液传感器;可调纳米复合界面; </div> </li> </ul> </div> </div> <div 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