Characterizing the Effects of a “Switchable Water” Additive on the Aqueous Solubility of Small Molecules

Vanderveen Jesse R.; Burra Sarika; Geng Jialing; Goyon Alexandre; Jardine Alexander; Shin Hyejin E.; Andrea Tamer; Dyson Paul J.; Jessop Philip G.

摘要

Abstract > “Switchable water” is an aqueous solution containing a water‐soluble amine additive that exhibits CO <sub>2</sub> ‐switchable properties, such as large changes in ionic strength, by forming an ammonium bicarbonate salt. Switchable water has been used to reversibly “salt‐out” organic compounds from water. This study explores the salting out of several compounds in switchable water when CO <sub>2</sub> is present and also explores the solubility of small molecules in switchable water, compared to pure water, when CO <sub>2</sub> is absent. The results show that organic compounds are generally more soluble in switchable water than pure water in the absence of CO <sub>2</sub> , but less soluble in the presence of 1?atm CO <sub>2</sub> . Exceptions include carboxylic acids and phenols which, presumably due to their acidity, are more soluble in switchable water than in pure water, even when CO <sub>2</sub> is applied. Kirkwood–Buff solvation theory was applied to gain insights into the effects of the amine additive on the aqueous solubility of caffeine. Furthermore, the switchable properties of the additives allow for the preparation of switchable aqueous two‐phase systems. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>摘要</标题> >“可切换水”是含有水溶性胺添加剂的水溶液，其表现出CO <通过形成碳酸氢铵盐，亚次> 2 </ sub> - 开关性质，例如离子强度的大变化。可切换的水已被用于可逆地从水中的“盐分”有机化合物。当存在CO <sub> 2 </ sub>时，该研究探讨了可切换水中的几种化合物中的盐分，并且在CO <SUB> 2 <sub时，与纯净水相比，在可切换水中探讨了小分子在可切换水中的溶解度。 >不存在。结果表明，在不存在CO <sub> 2 </ sub>的情况下，有机化合物通常比纯水更易溶于可切换水，但在1〜ATM CO <sub> 2 </ sub>存在下易溶。例外包括羧酸和酚，其可能由于它们的酸度而言，在施加CO <sub> 2 </ sub>时，即使在纯水中也比在纯水中溶于可切换水。应用柯克伍德 - 抗抗溶剂化理论，以获得胺添加剂对咖啡因含水溶解度的影响。此外，添加剂的可切换性质允许制备可切换的水性两相系统。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16300/'>《Chemphyschem: A European journal of chemical physics and physical chemistry》</a> <b style="margin: 0 2px;">|</b><span>2018年第16期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Vanderveen Jesse R.&option=202" target="_blank" rel="nofollow">Vanderveen Jesse R.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Burra Sarika&option=202" target="_blank" rel="nofollow">Burra Sarika;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Geng Jialing&option=202" target="_blank" rel="nofollow">Geng Jialing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Goyon Alexandre&option=202" target="_blank" rel="nofollow">Goyon Alexandre;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jardine Alexander&option=202" target="_blank" rel="nofollow">Jardine Alexander;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shin Hyejin E.&option=202" target="_blank" rel="nofollow">Shin Hyejin E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Andrea Tamer&option=202" target="_blank" rel="nofollow">Andrea Tamer;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dyson Paul J.&option=202" target="_blank" rel="nofollow">Dyson Paul J.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jessop Philip G.&option=202" target="_blank" rel="nofollow">Jessop Philip G.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Institut des Sciences et Ingénierie Chimiquesécole Polytechnique Fédérale de Lausanne1015 Lausanne Switzerland;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> <p>Institut des Sciences et Ingénierie Chimiquesécole Polytechnique Fédérale de Lausanne1015 Lausanne Switzerland;</p> <p>Department of ChemistryQueen's UniversityKingston ON K7L 3N6 Canada;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aqueous two-phase systems&option=203" rel="nofollow">aqueous two-phase systems;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrotropy&option=203" rel="nofollow">hydrotropy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kirkwood–Buff theory&option=203" rel="nofollow">Kirkwood–Buff theory;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=solutions&option=203" rel="nofollow">solutions;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=switchable solvents&option=203" rel="nofollow">switchable solvents;</a> </p> <div class="translation"> 机译：两相系统;水溶性;Kirkwood-Buff理论;解决方案;可切换溶剂; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022115560.html">Characterizing the Effects of a “Switchable Water” Additive on the Aqueous Solubility of Small Molecules</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Vanderveen Jesse R.&option=202" target="_blank" rel="nofollow" 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2014</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-22635_thesis/02022672513.html">常用食品添加剂对水溶性红曲色素稳定性的影响</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵树欣&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 赵树欣</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=祁星博&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,祁星博</a> <span> <a href="/conference-cn-22635/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十届中国国际食品添加剂和配料展览会及研讨会 </a> <span> <span> . 2006</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020316359272.html">小分子添加剂对钙钛矿太阳能电池的性能影响研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=章锋&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 章锋</a> <span> . 2021</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061202943123.html">定量表征剪切效应对蜡晶聚集行为影响的试验装置及方法</a> <b>[P]</b> . <span> 中国专利： CN106872673B </span> <span> . 2018.06.29</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120109380014.html">定量表征剪切效应对蜡晶聚集行为影响的试验装置及方法</a> <b>[P]</b> . <span> 中国专利： CN106872673A </span> <span> . 2017-06-20</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130472787509.html">Use of water soluble electrolytes as additives in aqueous polyurethane dispersions and an aqueous polyurethane dispersion containing a water soluble electrolyte</a> <b>[P]</b> . <span> 外国专利：  EP0013440B2 </span> <span> . 1985-05-08</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：水溶性电解质在水性聚氨酯分散体和含有水溶性电解质的水性聚氨酯分散体中作为添加剂的用途 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130474896218.html">Use of water soluble electrolytes as additives in aqueous dispersions of synthetic materials and an aqueous dispersion of synthetic materials containing a water soluble electrolyte</a> <b>[P]</b> . <span> 外国专利：  US4401786A </span> <span> . 1983-08-30</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：水溶性电解质在合成材料的水分散体和含有水溶性电解质的合成材料的水分散体中作为添加剂的用途 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130475131278.html">USE OF WATER SOLUBLE ELECTROLYTES AS ADDITIVES IN AQUEOUS SYNTHETIC RESIN DISPERSIONS AND AN AQUEOUS SYNTHETIC RESIN DISPERSION CONTAINING A WATER SOLUBLE ELECTROLYTE</a> <b>[P]</b> . <span> 外国专利：  DE2964396D1 </span> <span> . 1983-01-27</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在水溶性合成树脂分散体中使用水溶性电解质作为添加剂，以及在含有水溶性电解质的水性合成树脂分散体中使用水溶性电解质 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022115560','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" 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