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首页> 外文期刊>ChemSusChem >1D WO3 Nanorods/2D WO3?x Nanoflakes Homojunction Structure for Enhanced Charge Separation and Transfer towards Efficient Photoelectrochemical Performance
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1D WO3 Nanorods/2D WO3?x Nanoflakes Homojunction Structure for Enhanced Charge Separation and Transfer towards Efficient Photoelectrochemical Performance

机译：1d WO3纳米棒/ 2D WO3？X纳米薄片同源结结构，用于增强电荷分离和转移到有效的光电化学性能

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Abstract > Designing and fabricating photoelectrodes with low carrier recombination, high carrier transfer, and high light‐capture capability is of great significance for achieving effective photoelectrochemical (PEC) water splitting. Herein, for the first time, 2D nonstoichiometric WO <sub> 3? x </sub> nanoflakes (NFs) were vertically grown by hydrothermal synthesis on 1D WO <sub>3</sub> nanorods (NRs) obtained by a hydrothermal method and high‐temperature annealing (HTA). In this 1D HTA‐WO <sub>3</sub> /2D WO <sub> 3? x </sub> photoanode, the 2D WO <sub> 3? x </sub> NFs with active areas could maximize light harvesting, and the unique 1D/2D homojunction structure could improve the carrier‐separation efficiency. At the same time, the 1D WO <sub>3</sub> NRs with high aspect ratio were more beneficial to charge transfer after HTA. As expected, the 1D HTA‐WO <sub>3</sub> /2D WO <sub> 3? x </sub> photoanode yielded an enhanced photocurrent density of 0.98?mA?cm ?2 at 1.23?V versus reversible hydrogen electrode, which is approximately 3.16?times that of pristine WO <sub>3</sub> . The improvement could be attributed to the synergistic effect of HTA and the homojunction structure in the 1D HTA‐WO <sub>3</sub> /2D WO <sub> 3? x </sub> photoanode, which could effectively improve carrier separation and transfer. Furthermore, this work may provide a promising strategy for the design and fabrication of semiconductor‐based photoelectrodes. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 设计和制造具有低载体重组，高载体转移和高光捕集能力的光电极具对于实现有效的光电化学（PEC）水分裂具有重要意义。在此，首次，2D非级别计数 <sub> 3？ x </ i> </ sub> 纳米薄饼（NFS）在1D WO上通过水热合成垂直生长 <sub> 3 </ sub> 通过水热法和高温退火（HTA）获得的纳米棒（NRS）。在这个1d hta-wo <sub> 3 </ sub> / 2d wo. <sub> 3？ x </ i> </ sub> photoanode，2d wo <sub> 3？ x </ i> </ sub> 具有有源区域的NFS可以最大限度地提高光收获，并且独特的1D / 2D同质结结构可以提高载体分离效率。同时，1D WO <sub> 3 </ sub> 具有高纵横比的NRS对HTA之后的电荷转移更有益。正如预期的那样，1D HTA-WO <sub> 3 </ sub> / 2d wo. <sub> 3？ x </ i> </ sub> PhotoNode产生了增强的光电流密度为0.98？ma？cm ？2 </ sup> 在1.23？V与可逆氢电极，约为3.16Ω·倍 <sub> 3 </ sub> 。改善可能归因于1D HTA-WO中的HTA和同质结结构的协同效应 <sub> 3 </ sub> / 2d wo. <sub> 3？ x </ i> </ sub> PhotoNode，可以有效地改善载波分离和转移。此外，这项工作可以提供关于基于半导体的光电极的设计和制造的有希望的策略。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16185/'>《ChemSusChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第24期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yanting&option=202" target="_blank" rel="nofollow">Li Yanting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Zhifeng&option=202" target="_blank" rel="nofollow">Liu Zhifeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ruan Mengnan&option=202" target="_blank" rel="nofollow">Ruan Mengnan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Zhengang&option=202" target="_blank" rel="nofollow">Guo Zhengang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Xifei&option=202" target="_blank" rel="nofollow">Li Xifei;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Materials Science and EngineeringTianjin Chengjian UniversityTianjin 300384 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin Chengjian UniversityTianjin 300384 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin Chengjian UniversityTianjin 300384 P. R. China;</p> <p>School of Materials Science and EngineeringTianjin Chengjian UniversityTianjin 300384 P. R. China;</p> <p>Institute of Advanced Electrochemical Energy &</p> <p>School of Materials Science and EngineeringXi'an University of TechnologyXi'an 710048 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=homojunctions&option=203" rel="nofollow">homojunctions;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrothermal synthesis&option=203" rel="nofollow">hydrothermal synthesis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanostructures&option=203" rel="nofollow">nanostructures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photoelectrochemistry&option=203" rel="nofollow">photoelectrochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=water splitting&option=203" rel="nofollow">water splitting;</a> </p> <div class="translation"> 机译：同性全调;水热合成;纳米结构;光电化学;水分裂; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:35:31</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" 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