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Various Current Responses of Single Silver Nanoparticle Collisions on a Gold Ultramicroelectrode Depending on the Collision Conditions

机译：根据碰撞条件，单一银纳米粒子碰撞对金超微电极上的各种电流响应

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Abstract >Collisions of silver nanoparticles (NPs) with a more electrocatalytic gold or platinum ultramicroelectrode (UME) surface have been observed by using an electrochemical method. Depending on the applied potential to the UME, the current response to the collision of Ag NPs on the UME resulted in various shape changes. A staircase decrease, a blip decrease, and a blip increase of the hydrazine oxidation current were obtained at an applied potential of 0.33, 0.80, and 1.3?V, respectively. Different collision behaviors of Ag NPs on the UME surface were suggested for each shape of current response. Ag NP attachment, which hindered the diffusion flux to the UME, caused a staircase decrease of the electrocatalytic current. Instantaneous blocking of the hydrazine oxidation by Ag NP collision and, following recovery of the current by means of oxidation of Ag NP, caused a blip decrease of the electrocatalytic current. The formation of a higher oxidation state of Ag on the Ag NP and its electrocatalytic hydrazine oxidation resulted in a blip increase of the electrocatalytic current. The analysis of the current response of a single NP collision experiment can be a useful tool to understand the various behaviors of NPs on the electrode surface. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >冲突通过使用电化学方法，已经观察到具有更多电催化金或铂超微电极（UME）表面的银纳米颗粒（NPS）。根据卷筒的施加电位，对梅子上的AG NP的碰撞的电流响应导致各种形状变化。在0.33,0.80和1.3Ωv的施加电位下，获得阶梯减少，粘合剂降低和肼氧化电流的膨胀增加。建议为每种电流响应形状提出了ume表面上Ag NP的不同碰撞行为。阻碍扩散通量的Ag NP附件导致电催化电流的楼梯减少。 Ag NP碰撞的肼氧化瞬时阻断，并通过Ag NP的氧化回收电流后，引起了电催化电流的膨胀降低。在Ag NP和其电催化肼氧化中形成较高氧化状态，导致电催化电流的膨胀增加。对单个NP碰撞实验的当前响应的分析可以是理解电极表面上NP的各种行为的有用工具。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16161/'>《Chemistry, an Asian journal》</a> <b style="margin: 0 2px;">|</b><span>2017年第18期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mun Seon Kyu&option=202" target="_blank" rel="nofollow">Mun Seon Kyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Sangmin&option=202" target="_blank" rel="nofollow">Lee Sangmin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Dong Young&option=202" target="_blank" rel="nofollow">Kim Dong Young;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kwon Seong Jung&option=202" target="_blank" rel="nofollow">Kwon Seong Jung;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryKonkuk University120 Neungdong-ro Gwangjin-gu Seoul 143-701 Korea;</p> <p>Department of ChemistryKonkuk University120 Neungdong-ro Gwangjin-gu Seoul 143-701 Korea;</p> <p>Department of ChemistryKonkuk University120 Neungdong-ro Gwangjin-gu Seoul 143-701 Korea;</p> <p>Department of ChemistryKonkuk University120 Neungdong-ro Gwangjin-gu Seoul 143-701 Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrochemistry&option=203" rel="nofollow">electrochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=gold&option=203" rel="nofollow">gold;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticles&option=203" rel="nofollow">nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=silver&option=203" rel="nofollow">silver;</a> </p> <div class="translation"> 机译：电殖分析;电化学;金;纳米粒子;银; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022087132.html">Various Current Responses of Single Silver Nanoparticle Collisions on a Gold Ultramicroelectrode Depending on the Collision Conditions</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mun Seon Kyu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Mun Seon Kyu,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Sangmin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Lee Sangmin,</a> <a 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