The Taming of the Maleimide: Fabrication of Maleimide‐Containing ‘Clickable’ Polymeric Materials

Oz Yavuz; Sanyal Amitav

摘要

Abstract >Functional polymers are widely employed in various areas of biomedical sciences. In order to tailor them for desired applications, facile and efficient functionalization of these polymeric materials under mild and benign conditions is important. Polymers containing reactive maleimide groups can be employed for such applications since they provide an excellent handle for conjugation of thiol‐ and diene‐containing molecules and biomolecules. Until recently, fabrication of maleimide containing polymeric materials has been challenging due to the interference from the highly reactive double bond. A Diels‐Alder/retro Diels‐Alder reaction sequence based strategy to transiently mask the maleimide group provides access to such polymeric materials. In this personal account, we summarize contributions from our group towards the fabrication and functionalization of maleimide‐containing polymeric materials over the past decade. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >功能聚合物广泛用于生物医学科学的各个领域。为了根据所需的应用来定制它们，在温和和良性条件下，这些聚合物材料的容易和有效的功能化是重要的。含有反应性马来酰亚胺基团的聚合物可用于这些应用，因为它们提供了含硫和二烯分子和生物分子的缀合的优异手柄。直到最近，由于来自高反应性双键的干扰，含有聚合物材料的马来酰亚胺的制备已经具有挑战性。基于Diels-ald / Ricro Diels-Alder反应序列对瞬时掩模的致致致致膜的策略提供对这种聚合物材料的途径。在这个个人账户中，我们在过去十年中总结了我们小组对含马来酰亚胺聚合物材料的制备和功能化的贡献。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16132/'>《Chemical record》</a> <b style="margin: 0 2px;">|</b><span>2018年第6期</span><b style="margin: 0 2px;">|</b><span>共17页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Oz Yavuz&option=202" target="_blank" rel="nofollow">Oz Yavuz;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sanyal Amitav&option=202" target="_blank" rel="nofollow">Sanyal Amitav;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryBogazici UniversityBebek 34342 Istanbul Turkey;</p> <p>Department of ChemistryBogazici UniversityBebek 34342 Istanbul Turkey;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Maleimide&option=203" rel="nofollow">Maleimide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Diels-Alder&option=203" rel="nofollow">Diels-Alder;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=retro Diels-Alder&option=203" rel="nofollow">retro Diels-Alder;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thiol-ene Click reaction&option=203" rel="nofollow">thiol-ene Click reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Post-polymerization modification&option=203" rel="nofollow">Post-polymerization modification;</a> </p> <div class="translation"> 机译：马来酰亚胺;Diels-Alder;retro Diels-Alder;硫醇-NE点击反应;聚合后改性; 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