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Sustainable synthesis of novel carbon microwires for the modification of a Ti mesh anode in bioelectrochemical systems

机译:可持续合成新型碳微丝,用于生物电化学系统中钛网阳极的改性

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摘要

Herein, an effective method was developed to integrate carbon microwires on Ti mesh (denoted as CM/TiM) to fabricate high-performance anodes with long-time stability in microbial fuel cell. CM/TiM was synthesized by colonizing filamentous fungi on the bread modified Ti mesh followed by carbonization, which could convert the attached mycelium into carbon microwires (denoted as CM). Benefiting from the biocompatibility and 3D interlaced structure of carbon microwires, the biomass accumulation (1027 +/- 83 mu g cm(-2)) of CM/TiM have been significantly improved nearly 3 folds, thus the fabricated CM/TiM demonstrated 2-fold higher current density (12.19 +/- 0.07 A m(-2)) with significantly increased stability compared with TiM. Therefore, the present high power output, chemical stability and hydrophilic carbon microwires make CM/TiM stable, scalable and environmentally sustainable anodes in bioelectrochemical systems. (C) 2019 Elsevier B.V. All rights reserved.
机译:在本文中,开发了一种有效的方法来将碳微丝集成在Ti网孔(表示为CM / TiM)上,以在微生物燃料电池中制造具有长期稳定性的高性能阳极。 CM / TiM的合成方法是,将丝状真菌定植在面包修饰的Ti网上,然后碳化,这可以将附着的菌丝体转化为碳微丝(表示为CM)。得益于碳微丝的生物相容性和3D交错结构,CM / TiM的生物量积累(1027 +/- 83μg cm(-2))已显着提高了近3倍,因此制造的CM / TiM表现出2-与TiM相比,具有更高的电流密度(12.19 +/- 0.07 A m(-2))并具有显着提高的稳定性。因此,当前的高功率输出,化学稳定性和亲水性碳微丝使生物化学系统中的CM / TiM稳定,可扩展且在环境上可持续。 (C)2019 Elsevier B.V.保留所有权利。

著录项

  • 来源
    《The Science of the Total Environment》 |2019年第15期|294-302|共9页
  • 作者单位

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

    Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Carbon microwires; Titanium mesh; Sustainable; Stable; Bioelectrochemical systems;

    机译:碳微丝钛网可持续稳定生物电化学系统;

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