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Room-temperature exciton-polaritons with two-dimensional WS2

机译:二维WS2的室温激子极化子

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摘要

Two-dimensional transition metal dichalcogenides exhibit strong optical transitions with significant potential for optoelectronic devices. In particular they are suited for cavity quantum electrodynamics in which strong coupling leads to polariton formation as a root to realisation of inversionless lasing, polariton condensation and superfluidity. Demonstrations of such strongly correlated phenomena to date have often relied on cryogenic temperatures, high excitation densities and were frequently impaired by strong material disorder. At room-temperature, experiments approaching the strong coupling regime with transition metal dichalcogenides have been reported, but well resolved exciton-polaritons have yet to be achieved. Here we report a study of monolayer WS2 coupled to an open Fabry-Perot cavity at room-temperature, in which polariton eigenstates are unambiguously displayed. In-situ tunability of the cavity length results in a maximal Rabi splitting of ħΩRabi = 70 meV, exceeding the exciton linewidth. Our data are well described by a transfer matrix model appropriate for the large linewidth regime. This work provides a platform towards observing strongly correlated polariton phenomena in compact photonic devices for ambient temperature applications.
机译:二维过渡金属二卤化物显示出很强的光学跃迁,对光电器件具有巨大的潜力。特别地,它们适用于腔量子电动力学,在腔量子电动力学中,强耦合导致极化子的形成,是实现无反转激光,极化子凝聚和超流的基础。迄今为止,此类强相关现象的论证常常依赖于低温,高激发密度,并且经常因强烈的物质紊乱而受到损害。在室温下,已经报道了用过渡金属二卤化物接近强耦合态的实验,但是尚未实现良好解析的激子-极化子。在这里,我们报告了在室温下耦合到开放Fabry-Perot腔的单层WS2的研究,其中清晰地显示了极化子本征态。腔长度的原位可调谐性导致最大拉比分裂为ħΩRabi= 70 meV,超过了激子线宽。我们的数据通过适用于大线宽区域的传输矩阵模型得到了很好的描述。这项工作为观察环境温度应用的紧凑型光子器件中的强相关极化现象提供了一个平台。

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