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Room-temperature Tamm-plasmon exciton-polaritons with a WSe2 monolayer

机译:具有WSe2单层的室温Tamm-等离子体激子激子-极化子

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摘要

Solid-state cavity quantum electrodynamics is a rapidly advancing field, which explores the frontiers of light–matter coupling. Metal-based approaches are of particular interest in this field, as they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit. Transition metal dichalcogenides are ideally suited as the active material in cavity quantum electrodynamics, as they interact strongly with light at the ultimate monolayer limit. Here, we implement a Tamm-plasmon-polariton structure and study the coupling to a monolayer of WSe2, hosting highly stable excitons. Exciton-polariton formation at room temperature is manifested in the characteristic energy–momentum dispersion relation studied in photoluminescence, featuring an anti-crossing between the exciton and photon modes with a Rabi-splitting of 23.5 meV. Creating polaritonic quasiparticles in monolithic, compact architectures with atomic monolayers under ambient conditions is a crucial step towards the exploration of nonlinearities, macroscopic coherence and advanced spinor physics with novel, low-mass bosons.
机译:固态腔量子电动力学是一个快速发展的领域,它探索了光-质耦合的前沿。基于金属的方法在该领域中特别受关注,因为它们具有将光学模式挤压到明显低于衍射极限的空间的潜力。过渡金属二卤化物非常适合用作腔量子电动力学中的活性材料,因为它们在极限单层极限下会与光发生强烈相互作用。在这里,我们实现了Tamm-等离激元-极化子结构,并研究了与包含高稳定激子的WSe2单层的耦合。室温下激子-极化子的形成表现在光致发光中的特征能量-动量色散关系中,其特征在于激子和光子模之间的反交叉,Rabi分裂为23.5 meV。在环境条件下,在具有原子单层的整体紧凑结构中创建极化子准粒子,是探索非线性,宏观相干性和具有新型低质量玻色子的先进旋子物理学的关键一步。

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