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Dynamically controlled Purcell enhancement of visible spontaneous emission in a gated plasmonic heterostructure

机译:动态控制的赛尔增强门控等离子体异质结构中可见自发发射的能力

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摘要

Emission control of colloidal quantum dots (QDs) is a cornerstone of modern high-quality lighting and display technologies. Dynamic emission control of colloidal QDs in an optoelectronic device is usually achieved by changing the optical pump intensity or injection current density. Here we propose and demonstrate a distinctly different mechanism for the temporal modulation of QD emission intensity at constant optical pumping rate. Our mechanism is based on the electrically controlled modulation of the local density of optical states (LDOS) at the position of the QDs, resulting in the modulation of the QD spontaneous emission rate, far-field emission intensity, and quantum yield. We manipulate the LDOS via field effect-induced optical permittivity modulation of an ultrathin titanium nitride (TiN) film, which is incorporated in a gated TiN/SiO2/Ag plasmonic heterostructure. The demonstrated electrical control of the colloidal QD emission provides a new approach for modulating intensity of light in displays and other optoelectronics.
机译:胶体量子点(QD)的发射控制是现代高质量照明和显示技术的基石。通常通过改变光泵浦强度或注入电流密度来实现光电器件中胶体量子点的动态发射控制。在这里,我们提出并证明了在恒定的光泵浦速率下对QD发射强度进行时间调制的截然不同的机制。我们的机制基于对量子点位置处的光学态局部密度(LDOS)的电控制调制,从而对量子点的自发发射速率,远场发射强度和量子产率进行了调制。我们通过场效应感应的超薄氮化钛(TiN)薄膜的介电常数调制来操纵LDOS,该薄膜被集成在门控TiN / SiO2 / Ag等离子体异质结构中。胶体量子点发射的已证明的电控制为调制显示器和其他光电器件中的光强度提供了一种新方法。

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