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Recent Advances in Carbonaceous Photocatalysts with Enhanced Photocatalytic Performances: A Mini Review

机译:具有增强的光催化性能的碳质光催化剂的最新进展:小型回顾。

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摘要

Photocatalytic processes based on various semiconductors have been widely utilized in different applications, with great potential for use in environmental pollution remediation and sustainable energy generation. However, critical issues, including low light adsorption capability, wide energy bandgap, and unsatisfactory physicochemical stability still seriously limit the practical applications of photocatalysts. As a solution, the introduction of carbonaceous materials with different structures and properties into a photocatalyst system to further increase the activity has attracted much research attention. This mini review surveys the related literatures and highlights recent progress in the development of carbonaceous photocatalysts, which include various metal semiconductors with activated carbon, carbon dots, carbon nanotubesanofibers, graphene, fullerene, and carbon sponges/aerogels. Moreover, graphitic carbon nitride is also discussed as a carbon-rich and metal-free photocatalyst. The recently developed synthesis strategies and proposed mechanisms underlying the photocatalytic activity enhancement for different applications are summarized and discussed. Finally, ongoing challenges and the developmental direction for carbonaceous photocatalysts are proposed.
机译:基于各种半导体的光催化工艺已广泛用于不同的应用中,在环境污染修复和可持续能源生产中具有巨大的潜力。然而,包括低的光吸收能力,宽的能带隙和不令人满意的物理化学稳定性在内的关键问题仍然严重地限制了光催化剂的实际应用。作为解决方案,将具有不同结构和性质的碳质材料引入光催化剂体系以进一步提高活性已经引起了许多研究关注。这份简短的综述对相关文献进行了调查,并重点介绍了碳质光催化剂的最新进展,其中包括具有活性炭的各种金属半导体,碳点,碳纳米管/纳米纤维,石墨烯,富勒烯和碳海绵/气凝胶。此外,石墨氮化碳还被讨论为富碳且无金属的光催化剂。总结和讨论了最近开发的合成策略和针对不同应用的光催化活性增强的潜在机理。最后,提出了碳质光催化剂的挑战和发展方向。

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