Intramolecular Vibrational Energy Redistribution Measured by Femtosecond Pump-Probe Experiments in a Hollow Waveguide

摘要

We report femtosecond pump-probe experiments to investigate the intramolecular vibrational energy redistribution in the gas phase for CF_3CHFI, CHBrFI, CHBrClF and benzene (C_6H_6). To increase the measured probe signal the experiments have been performed in a hollow waveguide.