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Mechanisms and dynamics of optical nonlinearities in semiconductor nanocrystals

机译:半导体纳米晶体中光学非线性的机理和动力学

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Abstract: In this paper, we discuss the dynamics of carrier recombination in semiconductor nanoparticles embedded in a glass matrix, forming the so-called semiconductor-doped glasses. We observe that carrier recombination may be made faster by photodarkening and, at high excitation intensity, by Auger processes. We also discuss the mechanisms of the resonant optical Kerr effect in these materials. It is shown to be comprised of a fast component due to free carriers in particles without traps and of a slow one due to trapped carriers in particles with traps. The figure of merit associated with the fast component decreases when the particle size decreases.!22
机译:摘要:在本文中,我们讨论了嵌入玻璃基质中的半导体纳米颗粒中载流子复合的动力学,从而形成了所谓的半导体掺杂玻璃。我们观察到,通过光暗化可以使载流子重组更快,而在高激发强度下,通过俄歇过程可以使载流子重组更快。我们还将讨论这些材料中共振光学克尔效应的机理。由于没有陷阱的颗粒中的自由载流子,它由快组分组成;由于带有陷阱的颗粒中的被捕获的载流子,它由慢组分组成。当粒度减小时,与快速组分相关的品质因数也会降低。!22

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