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Real-time metrology of self-assembled epitaxial quantum dots by RHEED

机译:RHEED自组装外延量子点的实时计量

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Over recent years self assembled epitaxial quantum dots have gained much interest due to their potential for the development of advanced photovoltaic devices and the ability to control and reproduce desired structural properties of quantum dots (QD's) during growth is a desirable feature toward exploiting the full potential of these devices. Here and within the context of the archetype InAs/GaAs quantum dot system we provide an in situ approach to the determination of quantum dots size based on calculated reflection high energy electron diffraction (RHEED) patterns. We report the experimental evidence for the existence of periodic intensity fringes along the RHEED chevron tails predicted earlier by the theoretical model. The calculated and observed RHEED intensity profiles are analyzed systematically for different QD heights. The periodicity of the intensity fringes is correlated to the average height of the quantum dots and the possibility of monitoring real time the evolution of dot height during the MBE/CBE growth of self assembled quantum dots is demonstrated. The methodology demonstrated here when combined with the real time RHEED information on the dot surface coverage and facet orientation thus provides a full metrology of self assembled quantum dots that could be in turn used to improve control and reproducibility during growth of quantum dot heterostructures and devices.
机译:近年来,由于自组装外延量子点具有开发先进光伏器件的潜力,并且在生长过程中控制和再现量子点(QD)的所需结构特性的能力是开发全部潜能的理想功能,因此备受关注这些设备。在此,在原型InAs / GaAs量子点系统的背景下,我们提供了一种基于计算的反射高能电子衍射(RHEED)模式确定量子点尺寸的原位方法。我们报告了沿理论模型预测的RHEED V形人字形尾部存在周期性强度条纹的实验证据。对于不同的QD高度,系统地分析了计算和观察到的RHEED强度曲线。强度条纹的周期性与量子点的平均高度相关,并证明了在自组装量子点的MBE / CBE生长期间实时监测点高度变化的可能性。当与点表面覆盖率和刻面方向的实时RHEED信息结合使用时,此处演示的方法可提供自组装量子点的完整度量,这些量子点又可用于改善量子点异质结构和器件生长过程中的控制和可重复性。

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