The present invention is a method of poles configuration with four poles inter-combination for marine electromagnetic surveying and acquisition. The method of the present invention adopts six horizontal electric field components with four poles inter-combination. The six horizontal electric field components are respectively constituted from tri-pins grounding electrodes of four poles pairwise. One of the pins of each of the tri-pins grounding electrodes and the pins of the other three tri-pins grounding electrodes mutually constitute the six horizontal electric field components. The data for electromagnetic field over time series are simultaneously recorded. The present invention effectively ensure that the electric field recording with an angle less than 22.5 degree to the activation direction is achieved regardless of the orientation of the acquisition station, and that the worst effective activation signal may reach 76.5% of that under collinear activation. It is ensured that the activation field source and the couple pole for recording the electric field are under strong coupling, the requirements on the orientation of the acquisition station and on the dragging direction and position of the activation field source in data acquisition are lowered, and loss of electromagnetic data is prevented.
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