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Spin Orbit Effects in the Electronic Transport Properties of Adsorbed Graphene Nanoribbons

机译:自旋轨道对吸附石墨烯纳米带电子输运性质的影响

摘要

Graphene has received great attention due to its exceptional properties, which include corners with zero effective mass, extremely large mobilities, this could render it the new template for the next generation of electronic devices. Furthermore it has weak spin orbit interaction because of the low atomic number of carbon atom in turn results in long spin coherence lengths. Therefore, graphene is also a promising material for future applications in spintronic devices - the use of electronic spin degrees of freedom instead of the electron charge. Graphene can be engineered to form a number of different structures. In particular, by appropriately cutting it one can obtain 1-D system -with only a few nanometers in width - known as graphene nanoribbon, which strongly owe their properties to the width of the ribbons and to the atomic structure along the edges. Those GNR-based systems have been shown to have great potential applications specially as connectors for integrated circuits. Impurities and defects might play an important role to the coherence of these systems. In particular, the presence of transition metal atoms can lead to significant spin-flip processes of conduction electrons. Understanding this effect is of utmost importance for spintronics applied design. In this work, we focus on electronic transport properties of armchair graphene nanoribbons with adsorbed transition metal atoms as impurities and taking into account the spin-orbit effect. Our calculations were performed using a combination of density functional theory and non-equilibrium Greens functions. Also, employing a recursive method we consider a large number of impurities randomly distributed along the nanoribbon in order to infer, for different concentrations of defects, the spin-coherence length.
机译:石墨烯因其卓越的性能而备受关注,其中包括有效质量为零的角,极大的迁移率,这可能使其成为下一代电子设备的新模板。此外,由于碳原子的原子序数低,它具有弱的自旋轨道相互作用,进而导致长的自旋相干长度。因此,石墨烯也是自旋电子器件未来应用的有前途的材料-使用电子自旋自由度代替电子电荷。可以设计石墨烯以形成许多不同的结构。特别地,通过适当地切割它,​​可以获得仅具有几纳米宽度的1-D系统,即石墨烯纳米带,其强烈地归因于带的宽度和沿边缘的原子结构。那些基于GNR的系统已被证明具有巨大的潜在应用,特别是作为集成电路的连接器。杂质和缺陷可能对这些系统的一致性起重要作用。特别是过渡金属原子的存在会导致导电电子发生明显的自旋翻转过程。了解这种效应对于自旋电子学应用设计至关重要。在这项工作中,我们集中于吸附有过渡金属原子作为杂质的扶手椅石墨烯纳米带的电子输运性质,并考虑了自旋轨道效应。我们的计算是结合使用密度泛函理论和非平衡Greens函数进行的。同样,采用递归方法,我们考虑了沿着纳米带随机分布的大量杂质,以便针对不同浓度的缺陷推断出自旋相干长度。

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