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Nonlinear optical emission and near-field enhancement effects in arrays of gold bowtie nano-antennas

机译:金领结纳米天线阵列的非线性光发射和近场增强效应

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摘要

This thesis investigates the effects of the large near-field intensity enhancements from periodic arrays of gold bowtie nano-antennas (BNAs) after illumination by laser light. Specifically, we focus on laser-induced damage, nonlinear optical emission, and a proof-of-concept for utilizing arrays of gold BNAs to enhance the forces in an optical trapping system. From FDTD simulations, the optical response of a single BNA is demonstrated to increase the local intensity by a factor of 1000 in the feed-gap region by using a periodic array. Because of the high near-field intensities, inherently weak nonlinear optical processes become enhanced, and we take advantage of these favorable conditions to investigate the dependence of second-harmonic generation and two-photon photoluminescence emission intensities with respect to the array periodicity and the incident polarization. A detrimental side-effect of the efficient radiative coupling to the incident light and high near-field intensities is laser-induced damage, which may alter the morphology of the BNA structures at sufficiently high laser fluences. A damage threshold is systematically determined in terms of irradiation time and average incident power after implementation of damage reduction measures including laser pulse-width optimization, a stochastic beam-scanning pattern, and the use of a chromium adhesion layer. Finally, the increased optical forces in a trapping system resulting from the field enhancement of arrays of BNAs is demonstrated. In addition, based on the exclusive behaviors of these types of systems, a new method of characterizing plasmonically enhanced optical traps is proposed.
机译:本文研究了金领结纳米天线(BNA)的周期性阵列在激光照射后的大近场强度增强的影响。具体来说,我们专注于激光诱导的损坏,非线性光学发射以及利用金BNA阵列增强光阱系统中的力的概念验证。通过FDTD模拟,通过使用周期阵列,单个BNA的光学响应被证明可以在馈送间隙区域将局部强度提高1000倍。由于高的近场强度,固有的弱非线性光学过程变得增强,并且我们利用这些有利条件来研究二次谐波产生和双光子光致发光发射强度与阵列周期和入射的相关性。偏振。有效辐射耦合到入射光和高近场强度的有害副作用是激光诱导的损伤,这可能会在足够高的激光注量下改变BNA结构的形态。在实施损害减少措施(包括激光脉冲宽度优化,随机束扫描模式和使用铬粘附层)后,根据辐照时间和平均入射功率系统确定损害阈值。最后,展示了由于BNA阵列的场增强而导致的诱捕系统中增加的光学力。另外,基于这些类型系统的排他性行为,提出了表征等离子体增强的光阱的新方法。

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  • 作者

    Ko Kaspar D.;

  • 作者单位
  • 年度 2011
  • 总页数
  • 原文格式 PDF
  • 正文语种 {"code":"en","name":"English","id":9}
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