Chlorine-36 investigations of groundwater infiltration in the Exploratory Studies Facility at Yucca Mountain, Nevada

摘要

Chlorine-36, including the natural cosmogenic component and the component produced during atmospheric nuclear testing in the 1950`s and 1960`s (bomb pulse), is being used as an isotopic tracer for groundwater infiltration studies at Yucca Mountain, a potential nuclear waste repository. Rock samples have been collected systematically in the Exploratory Studies Facility (ESF), and samples were also collected from fractures, faults, and breccia zones. Isotopic ratios indicative of bomb-pulse components in the water ({sup 36}Cl/Cl values > 1,250 x 10{sup {minus}15}), signifying less than 40-yr travel times from the surface, have been detected at a few locations within the Topopah Spring Tuff, the candidate host rock for the repository. The specific features associated with the high {sup 36}Cl/Cl values are predominantly cooling joints and syngenetic breccias, but most of the sites are in the general vicinity of faults. The non-bomb pulse samples have {sup 36}Cl/Cl values interpreted to indicate groundwater travel times of at least a few thousand to possibly several hundred thousand years. Preliminary numerical solute-travel experiments using the FEHM (Finite Element Heat and Mass transfer) code demonstrate consistency between these interpreted ages and the observed {sup 36}Cl/Cl values but do not validate the interpretations.