Investigating the impact of regional transport on PM2.5 formation using vertical observation during APEC 2014 Summit in Beijing

摘要

During the APEC (Asia-Pacific Economic Cooperation) Economic Leaders' 2014 Summit in Beijing, strict regional air emission controls were implemented, providing a unique opportunity to investigate the transport and formation mechanism of fine particulate matter (PM2.5). This study explores the use of vertical observation methods to investigate the influence of regional transport on PM2.5 pollution in Beijing before and during the APEC Summit. Vertical profiles of extinction coefficient, wind, temperature and relative humidity were monitored at a rural site on the border of Beijing and Hebei Province. Three PM2.5 pollution episodes were analyzed. In episode 1 (27 October to 1 November), regional transport accompanied by the accumulation of pollutants under unfavorable meteorological conditions led to the pollution. In episode 2 (2-5 November), pollutants left from episode 1 were retained in the boundary layer of the region for 2 days and then settled down to the surface, leading to an explosive increase of PM2.5. The regional transport of aged aerosols played a crucial role in the heavy PM2.5 pollution. In episode 3 (6-11 November), emissions from large point sources had been controlled for several days while primary emissions from diesel vehicles might have led to the pollution. It is found that ground-level observation of meteorological conditions and air quality could not fully explain the pollution process, while vertical parameters (aerosol optical properties, winds, relative humidity and temperature) improved the understanding of regional transport influence on heavy pollution processes. Future studies may consider including vertical observations to aid investigation of pollutant transport, especially during episodic events of rapidly increasing concentrations.