Resin‐Derived Ni3S2/Carbon Nanocomposite for Advanced Rechargeable Aqueous Zn‐Based Batteries

Xiao Xiang; Zhang Haozhe; Wu Weixing; Wang Chao; Wu Shijia; Zhong Guobin; Xu Kaiqi; Zeng Jie; Su Wei; Lu Xihong

摘要

Abstract > The exploration of high‐energy and stable cathode materials is highly desirable and challenging for the development of advanced Zn‐based batteries. In this work, a facile pyrolysis method is reported to synthetize Ni <sub>3</sub> S <sub>2</sub> /carbon nanocomposite as high‐performance cathode by employing ion exchange resin as a precursor. Attributing to the abundant active sites and enhanced conductivity from well binding between Ni <sub>3</sub> S <sub>2</sub> and carbon, a markedly high capacity of 234.3 mA h g ?1 is obtained for this Ni <sub>3</sub> S <sub>2</sub> /carbon at a high current density of 6.9 A g ?1 . Moreover, a Zn‐based battery is demonstrated by using the Ni <sub>3</sub> S <sub>2</sub> /carbon as a cathode and Zn plate as an anode, which delivers a maximum power density of 58.6 kW kg ?1 , together with a peak energy density of 356 W h kg ?1 and 93.7% capacity retention after 5000 charging–discharging cycles. This simple synthetic strategy to achieve robust Ni‐based composite electrodes may open up new opportunities to design other transition metal–based electrodes for energy storage applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 高能量和稳定的阴极材料的探索是对先进的Zn基电池的开发非常理想和挑战。在这项工作中，将据报告一种容易的热解方法来综合NI <sub> 3 </ sub> S. <sub> 2 </ sub> /碳纳米复合材料通过使用离子交换树脂作为前体来高性能阴极。归因于丰富的活动位点，并在NI之间的良好结合中提高电导率 <sub> 3 </ sub> S. <sub> 2 </ sub> 和碳，高容量为234.3 ma h g ？1 </ sup> 获得了这个ni <sub> 3 </ sub> S. <sub> 2 </ sub> /碳的高电流密度为6.9 a g ？1 </ sup> 。此外，通过使用Ni证明了基于Zn的电池 <sub> 3 </ sub> S. <sub> 2 </ sub> /碳作为阴极和Zn板作为阳极，其发出58.6 kW kg的最大功率密度？1 </ sup> ，一起峰值能量密度为356 W H kg ？1 </ sup> 5000次充电循环后93.7％的容量保留。实现稳健的基于NI的复合电极的简单合成策略可以开辟新的机会，以设计用于储能应用的其他过渡金属基电极。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-28901/'>《Particle & Particle Systems Characterization: Measurement and Description of Particle Properties and Behavior in Powders and Other Disperse Systems 》</a> <b style="margin: 0 2px;">|</b><span>2019年第8期</span><b style="margin: 0 2px;">|</b> <span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xiao Xiang&option=202" target="_blank" rel="nofollow">Xiao Xiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Haozhe&option=202" target="_blank" rel="nofollow">Zhang Haozhe;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Weixing&option=202" target="_blank" rel="nofollow">Wu Weixing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Chao&option=202" target="_blank" rel="nofollow">Wang Chao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Shijia&option=202" target="_blank" rel="nofollow">Wu Shijia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhong Guobin&option=202" target="_blank" rel="nofollow">Zhong Guobin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Kaiqi&option=202" target="_blank" rel="nofollow">Xu Kaiqi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zeng Jie&option=202" target="_blank" rel="nofollow">Zeng Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Su Wei&option=202" target="_blank" rel="nofollow">Su Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Xihong&option=202" target="_blank" rel="nofollow">Lu Xihong;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>MOE of the Key Laboratory of Bioinorganic and Synthetic ChemistrySun Yat‐Sen UniversityGuangzhou 510275 P. R. China;</p> <p>MOE of the Key Laboratory of Bioinorganic and Synthetic ChemistrySun Yat‐Sen UniversityGuangzhou 510275 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>Electric Power Research Institute of Guangdong Power Grid Co. Ltd.Guangdong Guangzhou 510080 P. R. China;</p> <p>MOE of the Key Laboratory of Bioinorganic and Synthetic ChemistrySun Yat‐Sen UniversityGuangzhou 510275 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon composite&option=203" rel="nofollow">carbon composite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=high power density&option=203" rel="nofollow">high power density;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ni3S2&option=203" rel="nofollow">Ni3S2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=resin‐derived material&option=203" rel="nofollow">resin‐derived material;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zn‐based batteries&option=203" rel="nofollow">Zn‐based batteries;</a> </p> <div class="translation"> 机译：碳复合材料;高功率密度;Ni3S2;树脂衍生材料;Zn基电池; 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