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首页> 外文期刊>Materials science in semiconductor processing >One-step synthesis of Bi 2MoO 6/reduced graphene oxide aerogel composite with enhanced adsorption and photocatalytic degradation performance for methylene blue
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One-step synthesis of Bi 2MoO 6/reduced graphene oxide aerogel composite with enhanced adsorption and photocatalytic degradation performance for methylene blue

机译:双阶段合成BI 2 MOO 6 /减少石墨烯氧化物气凝胶复合材料,具有增强的吸附 亚甲蓝的光催化降解性能

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摘要

Bi2MoO6/reduced graphene oxide aerogel (BMO/GA) composite with enhanced adsorptivity and photocatalysis has been successfully synthesized through a simple one-step solvothermal method. During solvothermal synthesis, Bi2MoO6(BMO) as an efficient photocatalyst, which size was controllable, was uniformly distributed and well embedded into the pores of the 3D porous structure reduced graphene oxide aerogel (GA) and formed the 3D porous structure BMO/GA composite. The methylene blue (MB) was selected as a simulated pollutant, and the removal rate of BMO/GA composite toward MB was about 2.1 times as high as the pure BMO, which reached up 98.3% in 100?min. The BMO/GA composite with greatly improved adsorptivity and photocatalytic activity has some advantages of low-cost, ease of preparation and facile of recovery from target contaminant solution. The excellent adsorption and photocatalytic degradation performance of BMO/GA composite is mainly owing to the BMO can be exactly embedded into the pores of GA and the RGO provided conductive electron channels for dispersing electrons. The synergistic effect of BMO and GA on enhancing the adsorption and photocatalytic degradation toward MB was also discussed by a proposed photocatalytic mechanism.
机译:通过简单的一步溶剂热法成功地合成了Bi2Moo6 /氧化石墨烯氧化物气凝胶(BMO / GA)复合材料,具有增强的吸附性和光催化。在溶剂热合成期间,Bi2Moo6(BMO)作为一种有效的光催化剂,其尺寸是可控的,均匀地分布并充分地嵌入到3D多孔结构的孔中,还原氧化石墨烯氧化物气凝胶(GA)并形成3D多孔结构BMO / GA复合材料。选择亚甲基蓝(MB)作为模拟污染物,BMO / GA复合材料的去除率为MB的高度为纯BMO的约2.1倍,达到100μm的高达98.3%。具有大大提高的吸附性和光催化活性的BMO / GA复合材料具有低成本,易于准备和从靶污染物溶液中恢复的一些优点。 BMO / GA复合材料的优异吸附和光催化降解性能主要是由于BMO恰好嵌入到GA的孔中,并且RGO提供用于分散电子的导电电子通道。通过提出的光催化机制还讨论了BMO和GA对增强吸附和光催化降解的增强和光催化降解的协同作用。

著录项

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  • 作者单位

    Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University;

    Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University;

    Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University;

    The Key Laboratory of the Chinese Ministry of Education in Resource Chemistry Shanghai Normal University;

    Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University;

    Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 半导体技术 ;
  • 关键词

    Bi2MoO6/GA composite; Graphene aerogel; 3D porous structural; Photocatalytic degradation; Methylene blue;

    机译:Bi2moo6 / Ga复合;石墨烯气凝胶;3D多孔结构;光催化降解;亚甲基蓝色;

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