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A Global 3‐D Ocean Model for PCBs: Benchmark Compounds for Understanding the Impacts of Global Change on Neutral Persistent Organic Pollutants

机译：用于PCB的全球3-D海洋模型：用于了解全球变化对中性持久性有机污染物的影响的基准化合物

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Abstract >Human activities have released large quantities of neutral persistent organic pollutants (POPs) that may be biomagnified in food webs and pose health risks to wildlife, particularly top predators. Here we develop a global 3‐D ocean simulation for four polychlorinated biphenyls (PCBs) spanning a range of molecular weights and volatilities to better understand effects of climate‐driven changes in ocean biogeochemistry on the lifetime and distribution of POPs. Observations are most abundant in the Arctic Ocean. There, model results reproduce spatial patterns and magnitudes of measured PCB concentrations. Sorption of PCBs to suspended particles and subsequent burial in benthic marine sediment is the dominant oceanic loss process globally. Results suggest benthic sediment burial has removed 75% of cumulative PCB releases since the onset of production in 1930. Wind speed, light penetration, and ocean circulation exert a stronger and more variable influence on volatile PCB congeners with lower particle affinity such as chlorinated biphenyl‐28 and chlorinated biphenyl‐101. In the Arctic Ocean between 1992 and 2015, modeled evasion (losses) of the more volatile PCB congeners from the surface ocean increased due to declines in sea ice and changes in ocean circulation. By contrast, net deposition increased slightly for higher molecular weight congeners with stronger partitioning to particles. Our results suggest future climate changes will have the greatest impacts on the chemical lifetimes and distributions of volatile POPs with lower molecular weights. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><abstract type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >人类活动已发布大量的中性持续有机污染物（pops），可能是生物狼疮的食品网和对野生动物，特别是顶级掠夺者的健康风险。在这里，我们为四种多氯联苯（PCB）制定全球3-D海洋模拟，跨越一系列分子量和挥发性，以更好地理解气候驱动的变化在海洋生物地球化学中的寿命和分布的影响。观察在北冰洋中最丰富。在那里，模型结果再现空间模式和测量PCB浓度的大小。 PCB对悬浮颗粒的吸附和随后的底部沉积物之后的埋葬是全球主导海洋损失过程。结果表明，自1930年生产自爆发以来，底层沉积物埋葬已去除75％的累积PCB释放。风速，光渗透和海洋循环对具有较低粒子亲和力的挥发性PCB同一型，如氯化联苯 - 28和氯化双苯基-101。在1992年至2015年间，1992年至2015年间，由于海冰和海洋循环的变化，表面海洋的挥发性PCB同源物的建模逃避（损失）增加。相比之下，对于具有更强的分配给颗粒的更高分子量同一剂，净沉积略微增加。我们的结果表明，未来的气候变化将对较低分子量的化学生命混淆和挥发性污染物的分布产生最大的影响。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23728/'>《Global Biogeochemical Cycles》</a> <b style="margin: 0 2px;">|</b><span>2019年第3期</span><b style="margin: 0 2px;">|</b><span>共13页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wagner Charlotte C.&option=202" target="_blank" rel="nofollow">Wagner Charlotte C.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Amos Helen M.&option=202" target="_blank" rel="nofollow">Amos Helen M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Thackray Colin P.&option=202" target="_blank" rel="nofollow">Thackray Colin P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Yanxu&option=202" target="_blank" rel="nofollow">Zhang Yanxu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lundgren Elizabeth W.&option=202" target="_blank" rel="nofollow">Lundgren Elizabeth W.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Forget Gael&option=202" target="_blank" rel="nofollow">Forget Gael;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Friedman Carey L.&option=202" target="_blank" rel="nofollow">Friedman Carey L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Selin Noelle E.&option=202" target="_blank" rel="nofollow">Selin Noelle E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lohmann Rainer&option=202" target="_blank" rel="nofollow">Lohmann Rainer;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sunderland Elsie M.&option=202" target="_blank" rel="nofollow">Sunderland Elsie M.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> <p>Department of Earth Atmospheric and Planetary SciencesMassachusetts Institute of TechnologyCambridge MA USA;</p> <p>Corning School of Ocean StudiesMaine Maritime AcademyCastine ME USA;</p> <p>Institute for Data Systems and SocietyMassachusetts Institute of TechnologyCambridge MA USA;</p> <p>Graduate School of OceanographyUniversity of Rhode IslandNarragansett RI USA;</p> <p>Harvard John A. Paulson School of Engineering and Applied ScienceHarvard UniversityCambridge MA USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/165.html" title="地质学">地质学;</a><a href="https://www.zhangqiaokeyan.com/clc/5109.html" title="生物地球化学、气体地球化学">生物地球化学、气体地球化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ocean&option=203" rel="nofollow">ocean;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=biogeochemistry&option=203" rel="nofollow">biogeochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=persistent pollutants&option=203" rel="nofollow">persistent pollutants;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=fate and transport modeling&option=203" rel="nofollow">fate and transport modeling;</a> </p> <div class="translation"> 机译：海洋;生物地球化学;持续污染物;命运和运输建模; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023423671.html">A Global 3‐D Ocean Model for PCBs: Benchmark Compounds for Understanding the Impacts of Global Change on Neutral Persistent Organic Pollutants</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wagner Charlotte C.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Wagner Charlotte C.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Amos Helen M.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Amos Helen M.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Thackray Colin P.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Thackray Colin P.,</a> <a href="/journal-foreign-23728/" target="_blank" rel="nofollow" class="tuijian_authcolor">Global Biogeochemical Cycles .</a> <span>2019</span><span>,第3期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于PCB的全球3-D海洋模型：用于了解全球变化对中性持久性有机污染物的影响的基准化合物</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_detail_thesis/0204114688862.html">A review of ecological impacts of global climate change on persistent organic pollutant and mercury pathways and exposures in arctic marine ecosystems</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Melissa A. 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