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首页> 外文期刊>Advanced materials interfaces >Two‐Dimensional Titanium Carbide MXene as a Capacitor‐Type Electrode for Rechargeable Aqueous Li‐Ion and Na‐Ion Capacitor Batteries
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Two‐Dimensional Titanium Carbide MXene as a Capacitor‐Type Electrode for Rechargeable Aqueous Li‐Ion and Na‐Ion Capacitor Batteries

机译：用于可充电水性锂离子和NA离子电容器电池的二维碳化物MXINE作为电容器型电极

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摘要

Abstract > To bridge the gap of the alkali‐metal‐ion (Li or Na) batteries and supercapacitors, hybrid devices called capacitor batteries are being designed, which are adaptive for large‐scale energy‐storage systems. Two‐dimensional transition‐metal carbide materials (MXene) with high electronic conductivities have become capable electrode materials for supercapacitors. Herein, Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> synthesized by selectively etching the Al layer from the Ti <sub>3</sub> AlC <sub>2</sub> presents a remarkable electrochemical performance as an electrode material for the supercapacitor with Li <sub>2</sub> SO <sub>4</sub> or Na <sub>2</sub> SO <sub>4</sub> aqueous electrolyte. It displays a capacitance of 243?F?g ?1 at a low current density of 100?mA?g ?1 with a capacitance retention of 95?% in the Li <sub>2</sub> SO <sub>4</sub> electrolyte, and a capacitance of 150?F?g ?1 at a low current density of 200?mA?g ?1 with a capacitance retention of 95?% in the Na <sub>2</sub> SO <sub>4</sub> electrolyte, which shows its potential application for capacitor batteries. Moreover, the LiMn <sub>2</sub> O <sub>4</sub> //Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> Li‐ion capacitor battery and MnO <sub>2</sub> //Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> Na‐ion capacitor battery are designed and assembled for the first time. Such rechargeable aqueous capacitor batteries display capable capacities, remarkable rate abilities, and excellent cycling performances, which further demonstrates that Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> is an outstanding capacitor‐type electrode material for capacitor batteries. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > 为了弥合碱金属离子（Li或Na）电池和超级电容器的间隙，正在设计称为电容器电池的混合装置，这对于大型能量存储系统为自适应。具有高电子电导率的二维过渡金属碳化物材料（MXENE）已经成为超级电容器的电极材料。在此，TI. <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> 通过选择性地蚀刻来自Ti的Al层来合成 <sub> 3 </ sub> alc. <sub> 2 </ sub> 具有显着的电化学性能作为具有LI的超级电容器的电极材料 <sub> 2 </ sub> 所以 <sub> 4 </ sub> 或na <sub> 2 </ sub> 所以 <sub> 4 </ sub> 水性电解质。它显示器电容为243？g？g ？1 </ sup> 低电流密度为100？ma？g ？1 </ sup> 李的电容保留为95？％ <sub> 2 </ sub> 所以 <sub> 4 </ sub> 电解质，电容为150≤f？g ？1 </ sup> 低电流密度为200？ma？g ？1 </ sup> 在NA中的电容保留为95？％ <sub> 2 </ sub> 所以 <sub> 4 </ sub> 电解质显示其电容器电池的潜在应用。而且，跛行 <sub> 2 </ sub> O. <sub> 4 </ sub> // ti. <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> 锂离子电容器和MNO <sub> 2 </ sub> // ti. <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> Na离子电容器电池首次设计和组装。这种可充电水电池的能力显示能力，显着的速度能力和优异的循环性能，进一步证明了TI <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> 是电容器电池的优秀电容器型电极材料。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第11期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Kai&option=202" target="_blank" rel="nofollow">Zhu Kai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Hongyu&option=202" target="_blank" rel="nofollow">Zhang Hongyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ye Ke&option=202" target="_blank" rel="nofollow">Ye Ke;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Wenbin&option=202" target="_blank" rel="nofollow">Zhao Wenbin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Jun&option=202" target="_blank" rel="nofollow">Yan Jun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Kui&option=202" target="_blank" rel="nofollow">Cheng Kui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Guiling&option=202" target="_blank" rel="nofollow">Wang Guiling;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Baofeng&option=202" target="_blank" rel="nofollow">Yang Baofeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Dianxue&option=202" target="_blank" rel="nofollow">Cao Dianxue;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> <p>Shuangdeng Group Company LimitedJiangyan Jiangsu 225500 China;</p> <p>Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin Heilongjiang 150001 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=MXene&option=203" rel="nofollow">MXene;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=supercapacitor&option=203" rel="nofollow">supercapacitor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=capacitor battery&option=203" rel="nofollow">capacitor battery;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aqueous battery&option=203" rel="nofollow">aqueous battery;</a> </p> <div class="translation"> 机译：MXENE;超级电容器;电容器电池;水电池; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" 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break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：二维碳化钒（MXene）作为钠离子电容器的正极</span> </p> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_electronic-engineering-product-world_thesis/0201292139617.html">异军突起的固体锂离子可充电电池——新出现的固体锂离子可充电电池与液体锂离子电池和镍基电池展开激烈竞争</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . </a> <span> <a href="/journal-cn-8707/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 电子产品世界 </a> </span> <span> . 1996</span><span>,第4期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_automobile-parts_thesis/0201286379067.html">"两高"水性可充电电池问世比锂离子电池更安全、更便宜</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵飞明&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵飞明</a> <span> <a href="/journal-cn-9245/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 新型炭材料 </a> </span> <span> . 2000</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-22757_thesis/02022701957.html">高比能量混合型水系锂离子电池/电容器的研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=夏永姚&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 夏永姚</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王永钢&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王永钢</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=罗加严&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,罗加严</a> <span> <a href="/conference-cn-22757/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第二十七届全国化学与物理电源学术年会 </a> <span> <span> . 2006</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020311771629.html">金属氧化物作为锂离子电池和超级电容器电极材料的研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡宁&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 胡宁</a> <span> . 2018</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120103732794.html">锂离子电池用电极材料、锂离子电容器用电极材料、电极、电池、电容器、电子设备、锂离子电池用电极材料的制造方法以及锂离子电容器用电极材料的制造方法</a> <b>[P]</b> . <span> 中国专利： CN111052467A </span> <span> . 2020-04-21</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061201941431.html">电极对干燥法、锂离子二次电池制造法、双电层电容器制造法、锂离子电容器制造法</a> <b>[P]</b> . <span> 中国专利： CN103109397B </span> <span> . 2016.02.24</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130500875336.html">A current collector using an aluminum porous body having a three-dimensional network, an electrode using the current collector and non-aqueous electrolyte battery, capacitor and lithium ion capacitor with non-aqueous electrolytic solution each using the electrode, and method for producing the electrode</a> <b>[P]</b> . <span> 外国专利： <!-- --> DE112012000901B4 </span> <span> . 2021-10-21</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：使用具有三维网络的铝多孔体的集电器，使用电极的具有非水电解质电池，电容器和锂离子电容器的电极，以及每个使用电极的非水电解液，以及用于制造电极的方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130406079320.html">3 POROUS ALUMINUM MEMBER HAVING THREE-DIMENSIONAL RETICULATED STRUCTURE COLLECTOR AND ELECTRODE USING POROUS ALUMINUM MEMBER METHOD OF MANUFACTURING ELECTRODE NON-AQUEOUS ELECTROLYTE BATTERY USING ELECTRODE AND CAPACITOR AND LITHIUM-ION CAPACITOR USING NON-AQUEOUS ELECTROLYTE SOLUTION</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR101809519B1 </span> <span> . 2017-12-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：3具有三维网状集电体和电极的多孔铝构件，采用多孔铝构件的方法，利用电极和电容器以及锂离子电池，制造电极非水电解质电池 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130408671860.html">3 POROUS ALUMINUM MEMBER HAVING THREE-DIMENSIONAL RETICULATED STRUCTURE COLLECTOR AND ELECTRODE USING POROUS ALUMINUM MEMBER METHOD OF MANUFACTURING ELECTRODE NON-AQUEOUS ELECTROLYTE BATTERY USING ELECTRODE AND CAPACITOR AND LITHIUM-ION CAPACITOR USING NON-AQUEOUS ELECTROLYTE SOLUTION</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR20170096228A </span> <span> . 2017-08-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：3具有三维网状集电体和电极的多孔铝构件，采用多孔铝构件的方法，利用电极和电容器以及锂离子电池，制造电极非水电解质电池 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022435617','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="" onclick="$('.journalsub-pop-up').hide()"> <p 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