Mesoporous Thin Films for Fluid Manipulation

Mercuri Magalí; Berli Claudio L. A.; Bellino Martín G.

摘要

Abstract >The ability to control nanoflows is critical to design and fabricate ever more versatile nanosystems. Scientists are currently interested in finding ways to handle fluid dynamics inside nanoporous networks, not only to increase our knowledge of fluidic behavior but also to develop novel nanodevices that have potential utility in applications ranging from diagnostics to the production of high‐value chemicals. Here, we demonstrate how fluid motion can be manipulated by controlling the coexisting infiltration and evaporation phenomena in mesoporous films. A versatile actuation approach through liquid–vapor dynamic modulation was developed by integrating mesoporous substrates with a thermoelectric cell. This actuation resulted in fast and reversible fluid displacements through the mesoporous matrix, which was achieved with relatively small temperature variations by controlled voltage inputs. The versatility of the strategy is demonstrated by tunable cycling of fluid imbibition and switched nanofluidic connection of liquids into the substrate. This novel nanoflow manipulator could be the basis for smart nanofluidic devices toward exciting applications in actuators, controlled pattern formations and release systems. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >控制纳米氟的能力对于设计和制造更通用的纳米系统至关重要。科学家们目前有兴趣找到处理纳米多孔网络内的流体动力学的方法，不仅可以提高流体行为的知识，还可以开发具有在从诊断到生产高价值化学品的应用中具有潜在效用的新型纳米型。这里，我们证明了通过控制中孔膜中的共存渗透和蒸发现象来操纵流体运动。通过将介孔基板与热电电池集成来开发通过液体蒸汽动态调制的多功能致动方法。这种致动导致通过中孔矩阵的快速和可逆的流体位移，通过受控电压输入具有相对较小的温度变化来实现。通过可调谐循环的流体吸收和切换液体的纳米流体连接到基材中的循环循环来证明该策略的多功能性。该新颖的纳米洛操纵器可以是智能纳米流体装置对致动器，控制图案形成和释放系统的兴奋应用的基础。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第24期</span><b style="margin: 0 2px;">|</b><span>共5页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mercuri Magalí&option=202" target="_blank" rel="nofollow">Mercuri Magalí;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Berli Claudio L. A.&option=202" target="_blank" rel="nofollow">Berli Claudio L. A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bellino Martín G.&option=202" target="_blank" rel="nofollow">Bellino Martín G.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Comisión Nacional de Energía AtómicaAv. Gral. Paz 1499 San Martín B1650KNA Argentina;</p> <p>INTEC (Universidad Nacional del Litoral‐CONICET)Predio CCT CONICET Santa FeRN 168 3000 Santa Fe Argentina;</p> <p>Comisión Nacional de Energía AtómicaAv. Gral. Paz 1499 San Martín B1650KNA Argentina;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=fluid manipulation&option=203" rel="nofollow">fluid manipulation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=mesoporous materials&option=203" rel="nofollow">mesoporous materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanofluidics&option=203" rel="nofollow">nanofluidics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thin films&option=203" rel="nofollow">thin films;</a> </p> <div class="translation"> 机译：流体操纵;中孔材料;纳米流体;薄膜; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434826.html">Mesoporous Thin Films for Fluid Manipulation</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mercuri Magalí&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Mercuri Magalí,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Berli Claudio L. 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