A Double Self‐Assembly Process for Versatile Reduced‐Graphene‐Oxide Layer Deposition and Conformal Coating on 3D Structures

Jia Guobin; Plentz Jonathan; Presselt Martin; Dellith Jan; Dellith Andrea; Patze Sophie; T?lle Folke Johannes; Mülhaupt Rolf; Andr? Gudrun; Falk Fritz; Dietzek Benjamin

摘要

Abstract > In this work, a double self‐assembly (DSA) process is demonstrated based on the surface interaction between graphene flakes (GFs) and surfactant molecules at water/air interface, leading to the formation of a stable and dense monolayer of graphene flakes (MGFs) floating on water surface. The thus prepared MGFs can be easily transferred onto various substrates almost independent of their surface wettability. During deposition both the GFs and excess surfactant molecules rearrange themselves in a self‐assembled way, so that optimal compression of the MGFs is ensured. Consequently, high performance deposition of MGFs can be easily achieved. The here‐reported process combines a fast, reliable, equipment‐free large‐area (75 cm 2 in this work) high performance MGFs deposition onto most substrates irrespective to their wettability. Moreover, the DSA process enables an excellent conformal coating of MGFs on 3D structures. Thus, this technology has the potential to pave the way to many large‐scale affordable applications of low‐cost graphene feedstocks. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在这项工作中，基于水/空气界面下石墨烯片（GFS）和表面活性剂分子之间的表面相互作用来证明双重自组装（DSA）工艺，导致形成稳定和致密的石墨烯片（MGFS ）漂浮在水面上。由此制备的MGF可以容易地转移到各种基板上，几乎与其表面润湿性无关。在沉积期间，GFS和过量的表面活性剂分子以自组装方式重新排列本身，从而确保了MGF的最佳压缩。因此，可以容易地实现MGF的高性能沉积。这里报道的过程结合了快速，可靠，无设备的大区域（＆ 75厘米 2 </ sup> 在这项工作中，与其润湿性无关，高性能MGFS沉积到大多数基材上。此外，DSA工艺能够在3D结构上使MGFS的优异共形涂层。因此，该技术有可能为低成本石墨烯原料的许多大规模实惠的应用铺平道路。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces 》</a> <b style="margin: 0 2px;">|</b><span>2017年第23期</span><b style="margin: 0 2px;">|</b> <span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jia Guobin&option=202" target="_blank" rel="nofollow">Jia Guobin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Plentz Jonathan&option=202" target="_blank" rel="nofollow">Plentz Jonathan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Presselt Martin&option=202" target="_blank" rel="nofollow">Presselt Martin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dellith Jan&option=202" target="_blank" rel="nofollow">Dellith Jan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dellith Andrea&option=202" target="_blank" rel="nofollow">Dellith Andrea;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Patze Sophie&option=202" target="_blank" rel="nofollow">Patze Sophie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=T?lle Folke Johannes&option=202" target="_blank" rel="nofollow">T?lle Folke Johannes;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mülhaupt Rolf&option=202" target="_blank" rel="nofollow">Mülhaupt Rolf;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Andr? Gudrun&option=202" target="_blank" rel="nofollow">Andr? Gudrun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Falk Fritz&option=202" target="_blank" rel="nofollow">Falk Fritz;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dietzek Benjamin&option=202" target="_blank" rel="nofollow">Dietzek Benjamin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Institute for Macromolecular ChemistryAlbert‐Ludwigs University FreiburgStefan‐Meier‐Str. 31 79104 Freiburg Germany;</p> <p>Institute for Macromolecular ChemistryAlbert‐Ludwigs University FreiburgStefan‐Meier‐Str. 31 79104 Freiburg Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> <p>Leibniz Institute of Photonic TechnologyAlbert‐Einstein‐Str. 9 07745 Jena Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=conformal deposition on 3D structures&option=203" rel="nofollow">conformal deposition on 3D structures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=convex and concave surfaces&option=203" rel="nofollow">convex and concave surfaces;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=double self‐assembly process&option=203" rel="nofollow">double self‐assembly process;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=large‐area monolayer of graphene flakes&option=203" rel="nofollow">large‐area monolayer of graphene flakes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=wettability&option=203" rel="nofollow">wettability;</a> </p> <div class="translation"> 机译：在3D结构上保全沉积;凸凹面;双重自组装过程;石墨烯片的大面积单层;润湿性; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-central-south-university_thesis/0201281771725.html">用于对称型超级电容器的自组装活性炭插层石墨烯膜</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=武圆圆&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">武圆圆,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=朱连文&option=202" 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