Conformal Carbon Nitride Coating as an Efficient Hole Extraction Layer for ZnO Nanowires‐Based Photoelectrochemical Cells

Hajduk ?pela; Berglund Sean P.; Podlogar Matejka; Dra?i? Goran; Abdi Fatwa F.; Orel Zorica C.; Shalom Menny

摘要

Abstract >Charge transfer at the semiconductor–electrolyte junction is one of the main challenges for further improvement of photoelectrochemical (PEC) water splitting cells due to the poor surface catalytic properties of most semiconductors for the water oxidation reaction. Here it is shown, for the first time, that a conformal and thin carbon nitride (CN) layer can efficiently extract holes from ZnO nanowires (NWs), leading to a great enhancement of both PEC performance and stability in alkaline solution. The conformal CN coating is acquired by using a new synthetic method which involves the deposition of small supramolecular assemblies on ZnO‐NWs as a seeding layer for the CN growth. Detailed PEC characterization reveals that the CN facilitates the hole transfer from the ZnO‐NWs to the electrolyte and acts as a protective shell, resulting in 3.5 times higher current densities and high external quantum efficiencies at 1.23 V versus RHE compared to the pristine ZnO‐NWs. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P>在半导体 - 电解质结处的电荷转移是由于大多数半导体的表面催化性质，用于水氧化反应的差，用于进一步改善光电化学（PEC）水分裂细胞的主要挑战之一。在这里，首次示出了共形和薄的碳氮（CN）层可以有效地从ZnO纳米线（NWS）中提取孔，从而大大提高了PEC性能和碱性溶液中的稳定性。通过使用新的合成方法获得共形CN涂层，所述合成方法涉及在ZnO-NW上沉积小超分子组件作为CN生长的播种层。详细的PEC表征揭示CN利用从ZnO-NWS到电解质的空穴传递并用作保护壳，导致电流密度为3.5倍，与原始ZnO-NWS相比，1.23V与Rhe为1.23V的外部量子效率。。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第24期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hajduk ?pela&option=202" target="_blank" rel="nofollow">Hajduk ?pela;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Berglund Sean P.&option=202" target="_blank" rel="nofollow">Berglund Sean P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Podlogar Matejka&option=202" target="_blank" rel="nofollow">Podlogar Matejka;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dra?i? Goran&option=202" target="_blank" rel="nofollow">Dra?i? Goran;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Abdi Fatwa F.&option=202" target="_blank" rel="nofollow">Abdi Fatwa F.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Orel Zorica C.&option=202" target="_blank" rel="nofollow">Orel Zorica C.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shalom Menny&option=202" target="_blank" rel="nofollow">Shalom Menny;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Materials ChemistryNational Institute of ChemistryHajdrihova 18 Ljubljana 1000 Slovenia;</p> <p>Helmholtz‐Zentrum Berlin für Materialien und Energie GmbHHahn‐Meitner‐Platz 1 Berlin 14109 Germany;</p> <p>Department for Nanostructured MaterialsJo?ef Stefan InstituteJamova c. 39 Ljubljana 1000 Slovenia;</p> <p>Department of Materials ChemistryNational Institute of ChemistryHajdrihova 18 Ljubljana 1000 Slovenia;</p> <p>Helmholtz‐Zentrum Berlin für Materialien und Energie GmbHHahn‐Meitner‐Platz 1 Berlin 14109 Germany;</p> <p>Department of Materials ChemistryNational Institute of ChemistryHajdrihova 18 Ljubljana 1000 Slovenia;</p> <p>Department of Colloid ChemistryMax Planck Institute of Colloids and InterfacesPotsdam 14424 Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon nitride&option=203" rel="nofollow">carbon nitride;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=conformal coating&option=203" rel="nofollow">conformal coating;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photoelectrochemical cell&option=203" rel="nofollow">photoelectrochemical cell;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=water oxidation&option=203" rel="nofollow">water oxidation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=zinc oxide nanowires&option=203" rel="nofollow">zinc oxide nanowires;</a> </p> <div class="translation"> 机译：氮化碳;保形涂层;光电化学电池;水氧化;氧化锌纳米线; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a 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<span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=黄紫洋&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 黄紫洋</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=梁广超&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,梁广超</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=范楼珍&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,范楼珍</a> <span> <a href="/journal-cn-10958/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 高等学校化学学报 </a> </span> <span> . 2011</span><span>,第011期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-south-china-normal-university-natural-science-edition_thesis/0201249762814.html">ZnO 纳米线与硫掺杂 TiO2微／纳复合材料的制备及其光催化活性</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张延霖&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张延霖</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=谢楚如&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,谢楚如</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=蔡文娟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,蔡文娟</a> <span> <a href="/journal-cn-4639/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 华南师范大学学报（自然科学版） </a> </span> <span> . 2016</span><span>,第001期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-9818_thesis/020222351773.html">有机-ZnO纳米线混合光电二极管特性</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李杰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李杰</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=蒋泉&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,蒋泉</a> <span> <a href="/conference-cn-9818/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2011年第三届全国光学青年学术会议 </a> <span> <span> . 2011</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314854458.html">基于ZnO纳米线阵列的光电化学电池型自供能紫外探测器的制备和研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=曾溢宇&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 曾溢宇</a> <span> . 2016</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061203500490.html">一种基于光场辐照发光和光电化学性能的Ag和ZnO复合纳米线材料及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN107604341B </span> <span> . 2019.10.01</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120110083706.html">一种基于光场辐照发光和光电化学性能的Ag和ZnO复合纳米线材料及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN107604341A </span> <span> . 2018-01-19</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130421694135.html">Optoelectronic light emitting device i.e. gallium nitride based LED, has p-doped planarized layer allowing radial injection of holes in nanowire, and n-type silicon substrate allowing axial injection of electrons in nanowire</a> <b>[P]</b> . <span> 外国专利：  FR2964796A1 </span> <span> . 2012-03-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：光电发光器件（即基于氮化镓的LED）具有p掺杂的平面化层，允许径向注入纳米线中的空穴，以及n型硅衬底，允许轴向注入纳米线中的电子 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130415411488.html">Method for producing p-type ZnO based compound semiconductor layer, method for producing ZnO based compound semiconductor element, p-type ZnO based compound semiconductor single crystal layer, ZnO based compound semiconductor element, and n-type ZnO based compound semiconductor laminate structure</a> <b>[P]</b> . <span> 外国专利：  US9064790B2 </span> <span> . 2015-06-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：p型ZnO基化合物半导体层的制造方法，ZnO基化合物半导体元件的制造方法，p型ZnO基化合物半导体单晶层，ZnO基化合物半导体元件和n型ZnO基化合物半导体层叠结构 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130418030636.html">METHOD FOR PRODUCING P-TYPE ZnO BASED COMPOUND SEMICONDUCTOR LAYER, METHOD FOR PRODUCING ZnO BASED COMPOUND SEMICONDUCTOR ELEMENT, P-TYPE ZnO BASED COMPOUND SEMICONDUCTOR SINGLE CRYSTAL LAYER, ZnO BASED COMPOUND SEMICONDUCTOR ELEMENT, AND N-TYPE ZnO BASED COMPOUND SEMICONDUCTOR LAMINATE STRUCTURE</a> <b>[P]</b> . <span> 外国专利：  US2014027766A1 </span> <span> . 2014-01-30</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：制备P型ZnO基复合半导体层的方法，制备ZnO基复合半导体元件的方法，P型ZnO基复合半导体，单晶层，ZnO基复合半导体粉体，ZnO </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022433679','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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