首页> 外文期刊>ChemElectroChem >Improving Stability of LiCoO2 Cathode by Using Lithium Bis(Trifluoroborane)‐5‐Cyano‐2‐(Trifluoromethyl) Benzimidazolide as Additive

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Improving Stability of LiCoO2 Cathode by Using Lithium Bis(Trifluoroborane)‐5‐Cyano‐2‐(Trifluoromethyl) Benzimidazolide as Additive

机译：通过使用锂双（三氟硼烷）-5-氰基-2-（三氟甲基）苯并咪唑啉代作为添加剂来提高LiCoO2阴极的稳定性

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Abstract > LiCoO <sub>2</sub> is an important cathode material of commercial lithium‐ion batteries (LIBs) and therefore, improving the stability when LiCoO <sub>2</sub> cathode is overcharged can have an immediate impact on commercial LIBs. A novel Li salt, lithium 5‐cyano‐bis(trifluoroborane)‐2‐(trifluoromethyl) benzimidazolide (Li[CBTBI]) is evidenced in this study as an effective additive for improving the electrode/electrolyte interface of LiCoO <sub>2</sub> at high voltage operation condition. The presence of 2?% additive in commercial 1?M LiPF <sub>6</sub> /EC+DEC lead to the formation of stable interface of LiCoO <sub>2</sub> through cycles to 4.5?V, as demonstrated in cyclic voltammetry (CV). Electrochemical impedance spectroscopy (EIS) indicates a low‐impedance of the formed interface in the presence of the additive. Cyclability test also shows an improved stability in overcharging potential window by the presence of 2?% additive. In situ diffuse reflectance infrared Fourier‐transformed spectroscopy (DRIFTS) confirms the suppression of LiPF <sub>6</sub> decomposition, delay of onset potential of solid electrolyte interphase (SEI) formation, and thin SEI comparing to that without the additive. The possible reasons of the advantageous effect of using Li salt additives are discussed. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 吉罗 <sub> 2 </ sub> 是商业锂离子电池（LIBS）的重要阴极材料，因此，加强LiCoO时的稳定性 <sub> 2 </ sub> 阴极过度充电会对商业自由人口产生直接影响。在本研究中证明了一种新的Li盐，5-氰基 - 双（三氟甲烷）-2-（三氟甲基）苯并咪唑酯（Li [Cbtbi]）作为改善LiCoO的电极/电解质界面的有效添加剂 <sub> 2 </ sub> 在高压操作条件下。在商业1？m lipf中存在2？％添加剂 <sub> 6 </ sub> / EC + DED导致了LiCo的稳定界面 <sub> 2 </ sub> 通过循环至4.5？v，如循环伏安法（CV）所示。电化学阻抗光谱（EIS）表示在添加剂存在下形成的界面的低阻抗。可行性测试还显示出通过2〜％添加剂的存在过度充电潜在窗口的改善稳定性。原位</ i> 漫反射红外傅里叶转化光谱（漂移）证实了LiPF的抑制 <sub> 6 </ sub> 分解，延迟固体电解质相互作用（SEI）形成的延迟，与没有添加剂的情况相比，薄的SEI比较。讨论了使用Li盐添加剂的有利效果的可能原因。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第22期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Admas Teshager Minbale&option=202" target="_blank" rel="nofollow">Admas Teshager Minbale;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Sheng‐Chiang&option=202" target="_blank" rel="nofollow">Yang Sheng‐Chiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hwang Bing‐Joe&option=202" target="_blank" rel="nofollow">Hwang Bing‐Joe;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Shawn D.&option=202" target="_blank" rel="nofollow">Lin Shawn D.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical EngineeringNational Taiwan University of Science and Technology43 Keelung Road Sec.4 Taipei 106 Taiwan;</p> <p>Department of Chemical EngineeringNational Taiwan University of Science and Technology43 Keelung Road Sec.4 Taipei 106 Taiwan;</p> <p>Department of Chemical EngineeringNational Taiwan University of Science and Technology43 Keelung Road Sec.4 Taipei 106 Taiwan;</p> <p>Department of Chemical EngineeringNational Taiwan University of Science and Technology43 Keelung Road Sec.4 Taipei 106 Taiwan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrolyte additive&option=203" rel="nofollow">electrolyte additive;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=LiCoO2&option=203" rel="nofollow">LiCoO2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-ion batteries&option=203" rel="nofollow">lithium-ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=LiPF6&option=203" rel="nofollow">LiPF6;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=in?situ DRIFTS&option=203" rel="nofollow">in?situ DRIFTS;</a> </p> <div class="translation"> 机译：电解质添加剂;LiCoO2;锂离子电池;LiPF6;在呢？原位漂移; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:30:10</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022060508.html">Improving Stability of LiCoO2 Cathode by Using Lithium Bis(Trifluoroborane)‐5‐Cyano‐2‐(Trifluoromethyl) Benzimidazolide as Additive</a> <b>[J]</b> . <span> <a 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class="tuijian_authcolor"> . 第十四届全国农药信息交流会 </a> <span> <span> . 2006</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312843071.html">含2-三氟甲基苯并咪唑或三甲基硫阳离子化合物的合成及介电性质研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘明亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 刘明亮</a> <span> . 2014</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061201728436.html">4-[5-[3-氯-5-(三氟甲基)苯基]-4,5-二氢-5-(三氟甲基)-3-异噁唑基]-N-[2-氧代-2-[(2,2,2-三氟乙基)氨基]乙基]-1-萘甲酰胺的晶形</a> <b>[P]</b> . <span> 中国专利： CN102947278B </span> <span> . 2015.08.12</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120101637982.html">4-5-3-氯-5-(三氟甲基)苯基-4,5-二氢-5-(三氟甲基)-3-异*唑基-N-2-氧代-2-(2,2,2-三氟乙基)氨基乙基-1-萘甲酰胺的晶形</a> <b>[P]</b> . <span> 中国专利： CN102947278A </span> <span> . 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