Decanuclear Fe-III clusters with hemiacetal ligands: a new {M-10(mu(3)-O)(8)} cluster core

Mayans J.; Roc L.; Font-Bardia M.; Escuer A.

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Decanuclear Fe-III clusters with hemiacetal ligands: a new {M-10(mu(3)-O)(8)} cluster core

机译：具有半缩醛配体的Decanuclear Fe-III簇：新的{M-10（mu（3）-o）（8）}群体核心

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The characterization of a decanuclear Fe-III cluster with alpha-methyl-2-pyridinemethanolate, generated by the hydrolysis of Schiff bases, inspired us to carry out an initial exploration of the direct syntheses of medium nuclearity Fe-III clusters starting from aldehydes in methanolic medium. The new complexes exhibit an unprecedented {Fe-10(mu(3)-O)(8)} cluster core.

机译：通过Schiff碱的水解产生的α-甲基-2-吡啶蛋白乙醇酸酯的Decanumet Fe-III-III族蛋白的表征激发了美国从甲烷酚的醛开始的媒体核核心二氧化碳簇的直接合成的初步探索中等的。新的复合物展示了一个前所未有的{Fe-10（mu（3）-o）（8）}群体核心。

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《Dalton transactions: An international journal of inorganic chemistry 》 |2019年第35期| 共4页
作者
Mayans J.; Roc L.; Font-Bardia M.; Escuer A.;
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Univ Barcelona Dept Quim Inorgan &

Organ Seccio Organ Marti i Franques 1-11 E-08028 Barcelona Spain;

Univ Barcelona Dept Quim Inorgan &

Organ Seccio Organ Marti i Franques 1-11 E-08028 Barcelona Spain;

Univ Barcelona Dept Mineral Cristal Log &

Diposits Minerals Sole i Sabaris 1-3 E-08028 Barcelona Spain;

Univ Barcelona Dept Quim Inorgan &

Organ Seccio Organ Marti i Franques 1-11 E-08028 Barcelona Spain;

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正文语种 eng
中图分类化学 ; 无机化学 ;
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1. Decanuclear Fe-III clusters with hemiacetal ligands: a new {M-10(mu(3)-O)(8)} cluster core [J] . Mayans J., Roc L., Font-Bardia M., Dalton transactions: An international journal of inorganic chemistry . 2019 ,第35期

机译：具有半缩醛配体的Decanuclear Fe-III簇：新的{M-10（mu（3）-o）（8）}群体核心
2. Ligand substitution and growth reactions with Ru3Se2 nido clusters. Coordination isomerism in [WRu3(mu(4)-Se)(2)(mu-CO)(4)(CO)(7)(L)] (L = phosphine ligand) and electrochemical behaviour of the Ru3MSe2 core clusters (M = Ru, W) in solution [J] . Belletti D, Graiff C, Pattacini R, Inorganica Chimica Acta . 2005 ,第1期

机译：Ru3Se2 nido簇的配体取代和生长反应。 [WRu3（mu（4）-Se）（2）（mu-CO）（4）（CO）（7）（L）]中的配位异构体（L =膦配体）和Ru3MSe2核心簇的电化学行为（M =溶液中的Ru，W）
3. New tetranuclear metal carboxylate clusters with the [M-4(mu(3)-O)(2)](8+) (M = Mn-III or Fe-III) cores: crystal structures and properties of [Mn4O2Cl2(O2CC6H3F2-3,5)(6)(py)(4)], [Fe4O2Cl2(O2CMe)(6)(bpy)(2)] and [NBu4n][Fe4O2(O2CMe)(7)(pic)(2)] [J] . Wemple MW., Vincent JB., McCusker JK., Journal of the Chemical Society, Dalton Transactions. Inorganic Chemistry . 1998 ,第4期

机译：具有[M-4（mu（3）-O）（2）]（8 +）（M = Mn-III或Fe-III）核的新四核金属羧酸盐簇：[Mn4O2Cl2（O2CC6H3F2- 3,5）（6）（py）（4）]，[Fe4O2Cl2（O2CMe）（6）（bpy）（2）]和[NBu4n] [Fe4O2（O2CMe）（7）（pic）（2）]
4. Ligand Binding Energies and Structural Isomerism Accompanying Phosphine Ligand Exchange on Cationic Gold Clusters [C] . Marshall R. Ligare, Jose U. Reveles, Grant Johnson, ASMS Conference on Mass Spectrometry and Allied Topics . 2016

机译：伴随膦配体在阳离子金簇上交换的配体结合能量和结构异构体
5. Mechanisms of electron transfer and hydrogen activation in selected triruthenium clusters with multiple bridging ligands. Part I. The attenuation of radical reactivity in triruthenium trihydrido(alkylidyne) clusters. Electrochemistry and kinetics of decomposition of the 47-electron cluster radical, via a disproportionation path. Part II. The activation of molecular hydrogen at transition metal centers via kinetics and mechanism of reversible oxidative addition of hydrogen across the metal-metal bond of (mu-hydrogen)(2)Ruthenium(3)(Carbon monoxide)(8)(mu-phosphorus(t-BU)(2))(2). [D] . Bierdeman, David John. 2000

机译：具有多个桥联配体的选定三钌簇中电子转移和氢活化的机理。第一部分。三氢三钌（亚烷基）簇中自由基反应性的减弱。通过歧化路径分解47电子簇自由基的电化学和动力学。第二部分通过（mu-hydrogen）（2）钌（3）（一氧化碳）（8）（mu-phosphorus（）的金属-金属键上氢的可逆氧化加成反应的动力学和机理激活过渡金属中心的分子氢t-BU）（2））（2）。
6. Retention of the Cluster Core Structure during Ligand Exchange Reactions of Carboxylato-Substituted Metal Oxo Clusters [O] . Johannes Kreutzer, Michael Puchberger, Christine Artner, -1

机译：羧基取代的金属氧簇的配体交换反应中簇核心结构的保留
7. Decanuclear FeIII clusters with hemiacetal ligands: a new {M10(μ3-O)8} cluster core [O] . J. Mayans, L. Roc, M. Font-Bardia, 2019

机译：具有半缩醛配体的Decanuclear Feiii簇：新的{M10（μ3-O）8}群体核心
8. Synthesis and Structure of the Trinuclear Palladium Cluster (Pd3(PEt3)3(Mu2-NPh)2(Mu2-NHPh))Cl, Containing Bridging Imido and Amido Ligands [R] . Lee, S. W., Trogler, W. C. 1990

机译：含有桥联亚氨基和酰氨基配体的三核钯簇（pd3（pEt3）3（mu2-Nph）2（mu2-NHph））Cl的合成和结构

Decanuclear Fe-III clusters with hemiacetal ligands: a new {M-10(mu(3)-O)(8)} cluster core

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