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首页> 外文期刊>Journal of Physics. Condensed Matter >Dissipative dynamics of charged polarons in organic molecules
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Dissipative dynamics of charged polarons in organic molecules

机译:带电极化子在有机分子中的耗散动力学

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Within a non-adiabatic dynamical method, we simulate charged polaron motion and dissociation in an organic molecule in the presence of dissipation. The dissipation, represented by damping, is introduced to investigate the influence of temperature on the mobility of carriers. We find that the velocity of the polaron has an inversely linear dependence on the damping, and hence the relationship between mobility and temperature is a power law, which is in agreement with the corresponding experiments. We also find that the velocity of the polaron exhibits a continuous dependence on the electric field in the presence of dissipation. In addition, we find that, in the presence of dissipation, the critical field that dissociates a polaron is reduced
机译:在非绝热动力学方法中,我们在存在耗散的情况下模拟有机分子中的带电极化子运动和解离。引入以阻尼为代表的耗散量,以研究温度对载流子迁移率的影响。我们发现极化子的速度与阻尼成反比线性关系,因此迁移率和温度之间的关系是幂律,这与相应的实验一致。我们还发现,在存在耗散的情况下,极化子的速度表现出对电场的连续依赖性。此外,我们发现,在存在耗散的情况下,解离极化子的临界场会减小

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