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Optical absorption spectrum of rotated trilayer graphene

机译:旋转三层石墨烯的光吸收光谱

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摘要

Using ab initio calculations we have studied the optical linear response of different configurations of twisted trilayer graphene systems.Wehave found thatwhen one of the outer layers is rotated the system shows an angle-dependent optical spectrum as its twisted bilayer counterpart; however, in this case there are two absorption peaks located in the visible range of the spectrum and one more in the intermediate infrared range for large relative rotation angles. When two layers are rotated the spectrum exhibits only two absorption peaks in the visible range revealing information about the two relative rotation angles between the layers in the structure.All these absorption peaks in the visible range shift to the intermediate infrared range for small angles.
机译:使用从头算的方法,我们研究了扭曲的三层石墨烯系统不同构型的光学线性响应。我们发现,当外层之一旋转时,该系统会显示与角度相关的光谱作为扭曲的双层分子。但是,在这种情况下,对于较大的相对旋转角度,在光谱的可见范围内有两个吸收峰,在中红外范围内有一个吸收峰。当旋转两层时,光谱在可见光范围内仅显示两个吸收峰,揭示出结构中各层之间两个相对旋转角度的信息,所有这些可见光范围内的吸收峰都向小角度移动到中红外范围。

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