首页> 外文期刊>Journal of Nuclear Materials: Materials Aspects of Fission and Fusion >Damage and helium migration induced in fluorapatite sinters by swift heavy ion irradiations
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Damage and helium migration induced in fluorapatite sinters by swift heavy ion irradiations

机译:快速重离子辐照在氟磷灰石烧结物中引起的损伤和氦迁移

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摘要

We have studied the damage induced in fluorapatite (Ca _(10)(PO _4) _6F _2) sinters after 70-MeV Kr, 120 MeV I and 163-MeV Au ion irradiations at room temperature. On the basis of X-ray powder diffraction data we conclude that fluorapatite is not completely amorphized due to ion-induced recrystallization. This recrystallization of the amorphous phase is greatly enhanced for Au ions with a high electronic stopping power. We also have used the ~3He(d, p) ~4He nuclear reaction to study the migration of implanted 3-MeV ~3He ions after swift heavy ion irradiations. The proton yield curves versus deuteron energy for irradiated samples exhibit two bumps for high fluences. These excitation curves are deconvoluted by using a computer code based on a two-diffusion equation model of helium atoms in two accumulation zones. Optimizations of the model parameters give access to the diffusion coefficients and helium depth profiles in the two zones. This yields two broad peaks in the helium depth profiles, the first one is near the end-of-range region and the second one is shifted at about half way between the surface and the first peak. This shift is interpreted as a Radiation-Enhanced Diffusion (RED) effect which is found to increase with fluence for Kr ions, and with electronic stopping power from Kr to Au ions.
机译:我们已经研究了在室温下70 MeV Kr,120 MeV I和163 MeV Au离子辐照后在氟磷灰石(Ca _(10)(PO _4)_6F _2)烧结物中引起的损伤。根据X射线粉末衍射数据,我们得出结论,由于离子诱导的重结晶,氟磷灰石并未完全非晶化。对于具有高电子停止能力的Au离子,非晶相的这种重结晶得到了极大的增强。我们还使用〜3He(d,p)〜4He核反应来研究快速重离子辐照后注入的3-MeV〜3He离子的迁移。辐照样品的质子产率曲线与氘核能量的关系曲线显示出高通量有两个凸点。通过使用基于两个累积区中氦原子的二次扩散方程模型的计算机代码对这些激发曲线进行反卷积。通过优化模型参数,可以访问两个区域的扩散系数和氦深度剖面。这会在氦气深度剖面中产生两个宽峰,第一个在范围末端区域附近,第二个在表面和第一个峰之间移动了大约一半。该位移被解释为辐射增强扩散(RED)效应,发现该效应随Kr离子的通量以及从Kr到Au离子的电子阻止能力而增加。

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