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Effect of preparation methods on the performance of CeO2/Al2O3 catalysts for selective catalytic reduction of NO with NH3

机译:制备方法对CeO2 / Al2O3催化剂选择性催化NH3还原NO反应性能的影响

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摘要

CeO2/Al2O3 catalysts prepared by three methods were investigated for selective reduction of NO with NH3. It was found that the catalyst prepared by the single step sol-gel method had the best SCR activity and SO2 resistance performance. From the results of BET, XRD, TPD and TPR, it can be concluded that large surface area, strong interaction, highly dispersed nano-crystalline ceria, high NH3 adsorption capacity and good redox ability might be the main reasons for the excellent performance of CeO2/Al2O3 catalyst prepared by the single step sol-gel method.
机译:研究了用三种方法制备的CeO2 / Al2O3催化剂对NH3选择性还原NO的影响。发现通过单步溶胶-凝胶法制备的催化剂具有最佳的SCR活性和抗SO2性能。从BET,XRD,TPD和TPR的结果可以得出结论,大表面积,强相互作用,纳米晶体二氧化铈高度分散,高NH3吸附能力和良好的氧化还原能力可能是CeO2优异性能的主要原因。通过单步溶胶-凝胶法制备的/ Al2O3催化剂。

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