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Effect of voltage waveform on dielectric barrier discharge ozone production efficiency

机译:电压波形对介质阻挡放电臭氧产生效率的影响

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Dielectric barrier discharges (DBDs) are commonly used for gas effluent cleanup and ozone generation. For these applications, the energy efficiency of the discharge is a major concern. This paper reports on investigations carried out on the voltage shape applied to DBD reactor electrodes, aiming to evaluate a possible energy efficiency improvement for ozone production. Two DBD reactor geometries were used: pin-to-pin and cylinder-to-cylinder, both driven either by a bi-directional power supply (voltage rise rate 1 kV/μs) or by a pulsed power supply (voltage rise rate 1 kVs). Ozone formed in dry air was measured at the reactor outlet. Special attention was paid to discharge input power evaluation using different methods including instantaneous current-voltage product and transferred charge-applied voltage figures. The charge transferred by the discharges was also correlated to the ozone production. It is shown that, in the case of the DBD reactors under investigation, the applied voltage shape has no influence on the ozone production efficiency. For the considered voltage rise rate, the charge deposit on the dielectric inserted inside the discharge gap is the important factor (as opposed to the voltage shape) governing the efficiency of the discharge-it does this by tailoring the duration of the current peak into the tens of nanosecond range.
机译:介质阻挡放电(DBD)通常用于净化废气和产生臭氧。对于这些应用,放电的能量效率是一个主要问题。本文报告了对施加于DBD反应器电极的电压形状进行的研究,旨在评估可能提高臭氧生产效率的方法。使用了两种DBD反应器几何结构:引脚到引脚和圆柱到圆柱,两者均由双向电源(电压上升速率1 kV /μs)或脉冲电源(电压上升速率1 kV)驱动/ ns)。在反应器出口测量在干燥空气中形成的臭氧。要特别注意使用各种方法评估放电输入功率,包括瞬时电流-电压乘积和转移的电荷施加电压值。放电所转移的电荷也与臭氧的产生有关。结果表明,在所研究的DBD反应器中,所施加的电压形状对臭氧生产效率没有影响。对于所考虑的电压上升率,插入放电间隙内的电介质上的电荷沉积是控制放电效率的重要因素(与电压形状相反),这是通过将电流峰值的持续时间调整为适当的数十纳秒的范围。

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