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Low Mach number fluctuating hydrodynamics of multispecies liquid mixtures

机译:低马赫数波动的多种液体混合物的流体动力学

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We develop a low Mach number formulation of the hydrodynamic equations describing transport of mass and momentum in a multispecies mixture of incompressible miscible liquids at specified temperature and pressure, which generalizes our prior work on ideal mixtures of ideal gases [Balakrishnan et al., "Fluctuating hydrodynamics of multispecies nonreactive mixtures," Phys. Rev. E 89 013017 (2014)] and binary liquid mixtures [Donev et al., "Low mach number fluctuating hydrodynamics of diffusively mixing fluids," Commun. Appl. Math. Comput. Sci. 9(1), 47-105 (2014)]. In this formulation, we combine and extend a number of existing descriptions of multispecies transport available in the literature. The formulation applies to non-ideal mixtures of arbitrary number of species, without the need to single out a " solvent" species, and includes contributions to the diffusive mass flux due to gradients of composition, temperature, and pressure. Momentum transport and advective mass transport are handled using a low Mach number approach that eliminates fast sound waves (pressure fluctuations) from the full compressible system of equations and leads to a quasi-incompressible formulation. Thermal fluctuations are included in our fluctuating hydrodynamics description following the principles of nonequilibrium thermodynamics. We extend the semi-implicit staggered-grid finite-volume numerical method developed in our prior work on binary liquid mixtures [Nonaka et al., " Low mach number fluctuating hydrodynamics of binary liquid mixtures," arXiv:1410.2300 (2015)] and use it to study the development of giant nonequilibrium concentration fluctuations in a ternary mixture subjected to a steady concentration gradient. We also numerically study the development of diffusion-driven gravitational instabilities in a ternary mixture and compare our numerical results to recent experimental measurements [Carballido-Landeira et al., "Mixedmode instability of a miscible interface due to coupling between Rayleigh-Taylor and double-diffusive convective modes," Phys. Fluids 25, 024107 (2013)] in a Hele-Shaw cell. We find that giant nonequilibrium fluctuations can trigger the instability but are eventually dominated by the deterministic growth of the unstable mode, in both quasi-two-dimensional (Hele-Shaw) and fully three-dimensional geometries used in typical shadowgraph experiments. (C) 2015 AIP Publishing LLC.
机译:我们开发了一个低马赫数的流体力学方程式,描述了在特定温度和压力下不可压缩混溶液体的多种物种混合物中质量和动量的传输,从而推广了我们先前关于理想气体的理想混合物的工作[Balakrishnan等,“波动多种非反应性混合物的流体动力学”,物理。修订版E 89 013017(2014)]和二元液体混合物[Donev等,“扩散速度低的马赫数波动地影响扩散混合流体的流体动力学”,Commun。应用数学。计算科学9(1),47-105(2014)]。在这种表述中,我们结合并扩展了文献中有关多物种运输的现有描述。该配方适用于任意数量种类的非理想混合物,而无需单独选择“溶剂”种类,并且由于组成,温度和压力的梯度而对扩散质量通量有所贡献。动量传输和对流质量传输使用低马赫数方法处理,该方法从完全可压缩的方程组中消除了快速声波(压力波动),并导致了拟不可压缩的公式。遵循非平衡热力学原理,热波动包含在波动流体力学描述中。我们扩展了在我们先前对二元液体混合物的研究中开发的半隐式交错网格有限体积数值方法[Nonaka等人,“二元液体混合物的低马赫数波动流体动力学”,arXiv:1410.2300(2015)]和使用研究在稳定浓度梯度下的三元混合物中巨大的非平衡浓度波动的发展。我们还对三元混合物中由扩散驱动的重力不稳定性的发展进行了数值研究,并将我们的数值结果与最近的实验测量结果进行了比较[Carballido-Landeira等人,“由于瑞利-泰勒和双分子之间的耦合,混相界面的混合模式不稳定性。扩散对流模式”。流体25,024107(2013)]。我们发现,在典型的阴影图实验中使用的准二维(Hele-Shaw)和完全三维几何图形中,巨大的非平衡波动都可以触发不稳定性,但最终由不稳定模式的确定性增长决定。 (C)2015 AIP Publishing LLC。

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