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Comment On 'atomic Structure Model Of The Reconstructed Si(557) Surface With A Triple Step Structure: Adatom-parallel Dimer Model'

机译:评述“具有三步结构的重构Si(557)表面的原子结构模型:Adatom-parallel Dimer模型”

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摘要

Recently, [Oh et al. Phys. Rev. B 77, 155430 (2008)] reported on an atomic model for the so-called Si(557)-reconstructed surface with regular triple steps. The atomic structure model proposed was developed on the basis of high-resolution scanning tunneling microscopy (STM) images and first-principles calculations performed to match such STM images. Here we argue that the STM image presented is affected by an artifact, most likely related to a multiple tip image effect. Among other issues with the image presented, the corner holes for (7 × 7) reconstruction on Si(111) terraces are not visible, since a doubled image superimposed smears out such characteristic depression. The (×7) periodicity deduced for the edge facets, in contrast with previously reported STM images and electron-diffraction studies which unambiguously indicate a (×2) periodicity, arises from the same artifact. Finally, we remark that the (557) surface orientation and (112) orientation of triple steps assumed for first-principles calculations disregard the latest experimental data available, which suggests this surface has a (7 7 10) orientation and the steps in triple step do not form a well-defined plane [Surf. Sci. 600, 4878 (2006)].
机译:最近,[Oh等。物理Rev. B 77,155430(2008)]报道了具有规则三步法的所谓Si(557)重构表面的原子模型。提出的原子结构模型是在高分辨率扫描隧道显微镜(STM)图像和进行第一原理计算以匹配此类STM图像的基础上开发的。在这里,我们认为所呈现的STM图像受伪影的影响,最有可能与多尖端图像效果有关。在呈现的图像中,除其他问题外,在Si(111)平台上进行(7×7)重建的角孔不可见,因为叠加的双倍图像会涂抹这种特征性凹陷。与先前报道的STM图像和明确表明(×2)周期性的电子衍射研究相反,针对边缘小面推导的(×7)周期性是由同一伪像产生的。最后,我们注意到第一原理计算中假设的三步法的(557)面取向和(112)取向无视最新的可用实验数据,这表明该表面具有(7 7 10)取向,并且三步法中的台阶不要形成轮廓分明的平面[Surf。科学600,4878(2006)]。

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