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Polycyclic and organochlorine hydrocarbons in sediments of the northern South China Sea

机译:南海北部沉积物中的多环和有机氯烃

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摘要

We investigated the concentration distribution and composition of organic pollutants in sediments of the shelf and the deep northern South China Sea (NSCS). Concentrations of polycyclic aromatic hydrocarbons (Σ15PAH; 10.69–66.45 ng g−1), Dichlorodiphenyltrichloroethane (Σ4DDT; 0–0.82 ng g−1), and polychlorinated biphenyls (Σ24PCB; 0–0.12 ng g−1) are below established sediment quality guidelines, suggesting no environmental risk. Surprisingly, concentrations increase from the shelf to the deep NSCS, and are higher in the east of the study area. The organic pollutant composition indicates PAH mainly derived from pyrogenic sources, and mostly degraded DDT and PCB. However, in the deep NSCS, considerable contribution of petrogenic PAH, low chlorinated PCB and p,p′-DDT suggest more recent input from different sources compared to the shelf. From these results we infer that organic pollution in the NSCS does not originate from the Pearl River Estuary but from the NE SCS, SW of Taiwan.
机译:我们调查了架子和南海北部深部沉积物(NSCS)中有机污染物的浓度分布和组成。多环芳烃(Σ15PAH; 10.69–66.45 ng-1),二氯二苯基三氯乙烷(Σ4DDT; 0–0.82 ng-1)和多氯联苯(Σ24PCB; 0–0.12 ng-1)的浓度低于既定的沉积物质量准则,表明没有环境风险。出乎意料的是,浓度从架子到深层NSCS都增加了,而在研究区域的东部则更高。有机污染物成分表明PAH主要来自热源,大部分降解为DDT和PCB。然而,在深部NSCS中,成岩PAH,低氯化PCB和p,p'-DDT的大量贡献表明,与陆架相比,来自不同来源的更新投入更大。从这些结果可以推断出,NSCS中的有机污染不是源自珠江口,而是源自台湾西南部的NE SCS。

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