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Artifacts identification in apertureless near-field optical microscopy

机译:无孔近场光学显微镜中的伪像识别

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摘要

The aim of this paper is to provide criteria for optical artifacts recognition in reflection-mode apertureless scanning near-field optical microscopy, implementing demodulation techniques at higher harmonics. We show that optical images acquired at different harmonics, although totally uncorrelated from the topography, can be entirely due to far-field artifacts. Such observations are interpreted by developing the dipole-dipole model for the detection scheme at higher harmonics. The model, confirmed by the experiment, predicts a lack of correlation between the topography and optical images even for structures a few tens of nanometers high, due to the rectification effect introduced by the lock-in amplifier used for signal demodulation. Analytical formulas deduced for the far-field background permit to simulate and identify all the different fictitious patterns to be expected from metallic nanowires or nanoparticles of a given shape. In particular, the background dependence on the tip-oscillation amplitude is put forward as the cause of the error-signal artifacts, suggesting, at the same time, specific fine-tuning configurations for background-free imaging. Finally a careful analysis of the phase signal is carried out. In particular, our model correctly interprets the steplike dependence observed experimentally of the background phase signal versus the tip-sample distance, and suggests to look for smooth variations of the phase signal for unambiguous near-field imaging assessment.
机译:本文的目的是为反射模式无孔扫描近场光学显微镜中的光学伪像识别提供标准,在高谐波下实施解调技术。我们显示,尽管与地形完全不相关,但以不同谐波获取的光学图像可能完全归因于远场伪像。通过开发用于高次谐波检测方案的偶极子-偶极子模型来解释这些观察结果。经过实验验证的模型预测,由于用于信号解调的锁定放大器引入的整流效应,即使对于几十纳米高的结构,地形和光学图像之间也缺乏相关性。为远场背景推导的分析公式可以模拟和识别给定形状的金属纳米线或纳米粒子所期望的所有不同虚拟模式。特别地,提出了对尖端振荡幅度的背景依赖性作为误差信号伪像的原因,同时提出了无背景成像的特定微调配置。最后,对相位信号进行仔细分析。特别地,我们的模型正确地解释了实验观察到的背景相位信号相对于尖端样本距离的阶梯状相关性,并建议寻找相位信号的平滑变化以进行明确的近场成像评估。

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